Spin properties in droplet epitaxy-grown telecom quantum dots

Fuente: arXiv
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Auteurs principaux: Cizauskas, Marius, Sala, Elisa M., Heffernan, Jon, Fox, A. Mark, Bayer, Manfred, Greilich, Alex
Format: Preprint
Publié: 2025
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author Cizauskas, Marius
Sala, Elisa M.
Heffernan, Jon
Fox, A. Mark
Bayer, Manfred
Greilich, Alex
author_facet Cizauskas, Marius
Sala, Elisa M.
Heffernan, Jon
Fox, A. Mark
Bayer, Manfred
Greilich, Alex
contents We investigate the spin properties of InAs/InGaAs/InP quantum dots grown by metalorganic vapor-phase epitaxy (MOVPE) deposition using droplet epitaxy, which emit in the telecom C-band. Using pump-probe Faraday ellipticity measurements, we determine electron and hole $g$-factors of $|g_e| = 0.934$ and $|g_h| = 0.471$, with the electron $g$-factor being nearly twice as low as typical molecular beam epitaxy Stranski-Krastanov (SK) grown samples. Most significantly, we measure a longitudinal spin relaxation time $T_1 = 2.95\,μs$, representing an order of magnitude improvement over comparable MBE SK grown samples. Despite significant electron $g$-factor anisotropy, we observed that it is reduced relative to similar material composition samples grown with MBE or MOVPE SK methods. We attribute these g-factor anisotropy and spin lifetime improvements to the enhanced structural symmetry achieved via MOVPE droplet epitaxy, which mitigates the inherent structural asymmetry in strain-driven growth approaches for InAs/InP quantum dots. These results demonstrate that MOVPE droplet epitaxy-grown InAs/InGaAs/InP quantum dots exhibit favorable spin properties for potential implementation in quantum information applications.
format Preprint
id arxiv_https___arxiv_org_abs_2507_06058
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spin properties in droplet epitaxy-grown telecom quantum dots
Cizauskas, Marius
Sala, Elisa M.
Heffernan, Jon
Fox, A. Mark
Bayer, Manfred
Greilich, Alex
Mesoscale and Nanoscale Physics
We investigate the spin properties of InAs/InGaAs/InP quantum dots grown by metalorganic vapor-phase epitaxy (MOVPE) deposition using droplet epitaxy, which emit in the telecom C-band. Using pump-probe Faraday ellipticity measurements, we determine electron and hole $g$-factors of $|g_e| = 0.934$ and $|g_h| = 0.471$, with the electron $g$-factor being nearly twice as low as typical molecular beam epitaxy Stranski-Krastanov (SK) grown samples. Most significantly, we measure a longitudinal spin relaxation time $T_1 = 2.95\,μs$, representing an order of magnitude improvement over comparable MBE SK grown samples. Despite significant electron $g$-factor anisotropy, we observed that it is reduced relative to similar material composition samples grown with MBE or MOVPE SK methods. We attribute these g-factor anisotropy and spin lifetime improvements to the enhanced structural symmetry achieved via MOVPE droplet epitaxy, which mitigates the inherent structural asymmetry in strain-driven growth approaches for InAs/InP quantum dots. These results demonstrate that MOVPE droplet epitaxy-grown InAs/InGaAs/InP quantum dots exhibit favorable spin properties for potential implementation in quantum information applications.
title Spin properties in droplet epitaxy-grown telecom quantum dots
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2507.06058