Bulk spin-orbit torque-driven spin Hall nano-oscillators using PtBi alloys

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Main Authors: Shashank, Utkarsh, Kumar, Akash, Parvini, Tahereh Sadat, Heyen, Hauke, Zeng, Lunjie, Yankovich, Andrew B., Rajabali, Mona, Olsson, Eva, Münzenberg, Markus, Åkerman, Johan
Format: Preprint
Published: 2025
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author Shashank, Utkarsh
Kumar, Akash
Parvini, Tahereh Sadat
Heyen, Hauke
Zeng, Lunjie
Yankovich, Andrew B.
Rajabali, Mona
Olsson, Eva
Münzenberg, Markus
Åkerman, Johan
author_facet Shashank, Utkarsh
Kumar, Akash
Parvini, Tahereh Sadat
Heyen, Hauke
Zeng, Lunjie
Yankovich, Andrew B.
Rajabali, Mona
Olsson, Eva
Münzenberg, Markus
Åkerman, Johan
contents Spin-orbit-torque-driven auto-oscillations in spin Hall nano-oscillators (SHNOs) offer a transformative pathway toward energy-efficient, nanoscale microwave devices for next-generation neuromorphic computing and high-frequency technologies. A key requirement for achieving robust, sustained oscillations is reducing the threshold current ($I_{\text{th}}$), strongly governed by spin Hall efficiency ($θ_{\text{SH}}$). However, conventional strategies to enhance $θ_{\text{SH}}$ face trade-offs, including high longitudinal resistivity, interfacial effects, and symmetry-breaking torques that limit performance. Here, we demonstrate a substantial enhancement of the bulk spin Hall effect in PtBi alloys, achieving over a threefold increase in $θ_{\text{SH}}$, from 0.07 in pure Pt to 0.24 in Pt$_{94.0}$Bi$_{6.0}$ and 0.19 in Pt$_{91.3}$Bi$_{8.7}$, as extracted from DC-bias spin-torque ferromagnetic resonance. The enhanced $θ_{\text{SH}}$ originates from bulk-dominated, extrinsic side-jump scattering across all PtBi compositions. Correspondingly, we observe a 42\% and 32\% reduction in $I_{\text{th}}$ in 100 nm SHNOs based on Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{94.0}$Bi$_{6.0}$(4 nm) and Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{91.3}$Bi$_{8.7}$(4 nm), respectively. Structural characterization reveals reduced Pt crystallinity, along with emergence of preferred crystallographic orientations upon introducing higher Bi concentrations. Together, these results position PtBi alloys as a compelling alternative to conventional 5$d$ transition metals, enabling enhanced $θ_{\text{SH}}$ and significantly lower $I_{\text{th}}$, thus opening new avenues for energy-efficient neuromorphic computing and magnetic random access memory.
format Preprint
id arxiv_https___arxiv_org_abs_2507_10219
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Bulk spin-orbit torque-driven spin Hall nano-oscillators using PtBi alloys
Shashank, Utkarsh
Kumar, Akash
Parvini, Tahereh Sadat
Heyen, Hauke
Zeng, Lunjie
Yankovich, Andrew B.
Rajabali, Mona
Olsson, Eva
Münzenberg, Markus
Åkerman, Johan
Mesoscale and Nanoscale Physics
Applied Physics
Spin-orbit-torque-driven auto-oscillations in spin Hall nano-oscillators (SHNOs) offer a transformative pathway toward energy-efficient, nanoscale microwave devices for next-generation neuromorphic computing and high-frequency technologies. A key requirement for achieving robust, sustained oscillations is reducing the threshold current ($I_{\text{th}}$), strongly governed by spin Hall efficiency ($θ_{\text{SH}}$). However, conventional strategies to enhance $θ_{\text{SH}}$ face trade-offs, including high longitudinal resistivity, interfacial effects, and symmetry-breaking torques that limit performance. Here, we demonstrate a substantial enhancement of the bulk spin Hall effect in PtBi alloys, achieving over a threefold increase in $θ_{\text{SH}}$, from 0.07 in pure Pt to 0.24 in Pt$_{94.0}$Bi$_{6.0}$ and 0.19 in Pt$_{91.3}$Bi$_{8.7}$, as extracted from DC-bias spin-torque ferromagnetic resonance. The enhanced $θ_{\text{SH}}$ originates from bulk-dominated, extrinsic side-jump scattering across all PtBi compositions. Correspondingly, we observe a 42\% and 32\% reduction in $I_{\text{th}}$ in 100 nm SHNOs based on Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{94.0}$Bi$_{6.0}$(4 nm) and Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{91.3}$Bi$_{8.7}$(4 nm), respectively. Structural characterization reveals reduced Pt crystallinity, along with emergence of preferred crystallographic orientations upon introducing higher Bi concentrations. Together, these results position PtBi alloys as a compelling alternative to conventional 5$d$ transition metals, enabling enhanced $θ_{\text{SH}}$ and significantly lower $I_{\text{th}}$, thus opening new avenues for energy-efficient neuromorphic computing and magnetic random access memory.
title Bulk spin-orbit torque-driven spin Hall nano-oscillators using PtBi alloys
topic Mesoscale and Nanoscale Physics
Applied Physics
url https://arxiv.org/abs/2507.10219