Near transform-limited single photons from rapid-thermal annealed quantum dots

Fuente: arXiv
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Autori principali: Mannel, Hendrik, Rimek, Fabio, Zoellner, Marcel, Schwarz, Nico, Wieck, Andreas D., Bart, Nikolai, Ludwig, Arne, Geller, Martin
Natura: Preprint
Pubblicazione: 2025
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author Mannel, Hendrik
Rimek, Fabio
Zoellner, Marcel
Schwarz, Nico
Wieck, Andreas D.
Bart, Nikolai
Ludwig, Arne
Geller, Martin
author_facet Mannel, Hendrik
Rimek, Fabio
Zoellner, Marcel
Schwarz, Nico
Wieck, Andreas D.
Bart, Nikolai
Ludwig, Arne
Geller, Martin
contents Single-photon emitters are essential components for quantum communication systems, enabling applications such as secure quantum key distribution and the long-term vision of a quantum internet. Among various candidates, self-assembled InAs/GaAs quantum dots (QDs) remain highly promising due to their ability to emit coherent and indistinguishable photons, as well as their compatibility with photonic integration. In this work, we investigate the impact of post-growth rapid thermal annealing (RTA) on the quantum optical properties of single self-assembled QDs embedded in a p-i-n diode structure. The annealing process induces a controlled blueshift of the emission wavelength by promoting Ga in-diffusion and intermixing. Using resonance fluorescence measurements at cryogenic temperatures (4.2 K), we investigate the single-photon statistics, the emission linewidths, and coherence time $T_2$ of the emitted photons. Our results show that, despite the high annealing temperature of $760^\circ$C, the process does not degrade the optical quality of the quantum dots strongly. Instead, we observe single-photon emission with near transform-limited linewidths, where the dephasing time $T_2$ is only a factor 1.5 above the Fourier-limit $T_2=2T_1$. These findings demonstrate that rapid thermal annealing (RTA) serves as an effective tuning method that preserves the key single-photon emission properties and may help reduce undesirable effects such as non-radiative Auger recombination in quantum photonic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2507_11108
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Near transform-limited single photons from rapid-thermal annealed quantum dots
Mannel, Hendrik
Rimek, Fabio
Zoellner, Marcel
Schwarz, Nico
Wieck, Andreas D.
Bart, Nikolai
Ludwig, Arne
Geller, Martin
Mesoscale and Nanoscale Physics
Single-photon emitters are essential components for quantum communication systems, enabling applications such as secure quantum key distribution and the long-term vision of a quantum internet. Among various candidates, self-assembled InAs/GaAs quantum dots (QDs) remain highly promising due to their ability to emit coherent and indistinguishable photons, as well as their compatibility with photonic integration. In this work, we investigate the impact of post-growth rapid thermal annealing (RTA) on the quantum optical properties of single self-assembled QDs embedded in a p-i-n diode structure. The annealing process induces a controlled blueshift of the emission wavelength by promoting Ga in-diffusion and intermixing. Using resonance fluorescence measurements at cryogenic temperatures (4.2 K), we investigate the single-photon statistics, the emission linewidths, and coherence time $T_2$ of the emitted photons. Our results show that, despite the high annealing temperature of $760^\circ$C, the process does not degrade the optical quality of the quantum dots strongly. Instead, we observe single-photon emission with near transform-limited linewidths, where the dephasing time $T_2$ is only a factor 1.5 above the Fourier-limit $T_2=2T_1$. These findings demonstrate that rapid thermal annealing (RTA) serves as an effective tuning method that preserves the key single-photon emission properties and may help reduce undesirable effects such as non-radiative Auger recombination in quantum photonic applications.
title Near transform-limited single photons from rapid-thermal annealed quantum dots
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2507.11108