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Main Authors: Kuroda, Rin, Hughes, Vernon M., Poitrinal, Martin, Peper, Michael, Thompson, Jeff D.
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2507.11487
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author Kuroda, Rin
Hughes, Vernon M.
Poitrinal, Martin
Peper, Michael
Thompson, Jeff D.
author_facet Kuroda, Rin
Hughes, Vernon M.
Poitrinal, Martin
Peper, Michael
Thompson, Jeff D.
contents The complex Rydberg structure of ytterbium atoms is shaped by multiple low-lying ion-core-excited states and strong channel interactions, which presents both opportunities and challenges for quantum information processing and precision metrology. In this work, we extend high-resolution microwave spectroscopy and multichannel quantum defect theory (MQDT) modeling of singly excited $6sn\ell$ Rydberg states in $^{174}$Yb and $^{171}$Yb to include the $\ell = 3$ ($f$) and $\ell = 4$ ($g$) series. Our measurements reveal $p$-$f$ mixing in odd-parity Rydberg states of $^{171}$Yb, which we incorporate by combined MQDT models for $6snp$ and $6snf$ series. Additionally, we observe that for $\ell = 4$ the spin-orbit interaction dominates over the exchange interaction, such that the $6sng$ states are more accurately described in a $jj$-coupled basis. We validate our models by comparing the predicted Landé $g$-factors and static dipole polarizabilities with experimental measurements, finding excellent agreement. These results provide important input for designing high-fidelity entangling gates with ytterbium atoms.
format Preprint
id arxiv_https___arxiv_org_abs_2507_11487
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Microwave spectroscopy and multi-channel quantum defect analysis of ytterbium Rydberg states
Kuroda, Rin
Hughes, Vernon M.
Poitrinal, Martin
Peper, Michael
Thompson, Jeff D.
Atomic Physics
Quantum Physics
The complex Rydberg structure of ytterbium atoms is shaped by multiple low-lying ion-core-excited states and strong channel interactions, which presents both opportunities and challenges for quantum information processing and precision metrology. In this work, we extend high-resolution microwave spectroscopy and multichannel quantum defect theory (MQDT) modeling of singly excited $6sn\ell$ Rydberg states in $^{174}$Yb and $^{171}$Yb to include the $\ell = 3$ ($f$) and $\ell = 4$ ($g$) series. Our measurements reveal $p$-$f$ mixing in odd-parity Rydberg states of $^{171}$Yb, which we incorporate by combined MQDT models for $6snp$ and $6snf$ series. Additionally, we observe that for $\ell = 4$ the spin-orbit interaction dominates over the exchange interaction, such that the $6sng$ states are more accurately described in a $jj$-coupled basis. We validate our models by comparing the predicted Landé $g$-factors and static dipole polarizabilities with experimental measurements, finding excellent agreement. These results provide important input for designing high-fidelity entangling gates with ytterbium atoms.
title Microwave spectroscopy and multi-channel quantum defect analysis of ytterbium Rydberg states
topic Atomic Physics
Quantum Physics
url https://arxiv.org/abs/2507.11487