Metal-Insulator transition and Charge Transport Mechanisms in SnSe$_2$ Field-Effect Transistor

Fuente: arXiv
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Autores principales: Lakhara, Aarti, Thole, Lars, Haug, Rolf J., Bhobe, P. A.
Formato: Preprint
Publicado: 2025
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author Lakhara, Aarti
Thole, Lars
Haug, Rolf J.
Bhobe, P. A.
author_facet Lakhara, Aarti
Thole, Lars
Haug, Rolf J.
Bhobe, P. A.
contents We report an observation of metal-insulator transition in a thin film of SnSe$_2$. The room-temperature carrier concentration of SnSe$_2$ film was increased by electrostatic doping to 1.14$\times$ 10$^{13}$ cm$^{-2}$. A crossover from insulating phase to metallic state was clearly observed. The low-temperature charge transport mechanism is governed by two-dimensional (2D) variable-range hopping. This mechanism is influenced by band bending and gap states introduced by selenium vacancies. At low temperatures, the mobility is primarily limited by charged impurities, while at higher temperatures, it follows a power-law dependence, $μ= T^{-γ}$, indicating a dominance of electron-phonon scattering. The application of a gate field shifts the Fermi level toward the conduction band, and at sufficiently high temperatures, this drives the system into a metallic state. Our findings offer insights into the charge transport mechanisms in SnSe$_2$ FET, this understanding will allow for the optimization of other 2D materials for advanced electronic device applications.
format Preprint
id arxiv_https___arxiv_org_abs_2507_14536
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Metal-Insulator transition and Charge Transport Mechanisms in SnSe$_2$ Field-Effect Transistor
Lakhara, Aarti
Thole, Lars
Haug, Rolf J.
Bhobe, P. A.
Materials Science
We report an observation of metal-insulator transition in a thin film of SnSe$_2$. The room-temperature carrier concentration of SnSe$_2$ film was increased by electrostatic doping to 1.14$\times$ 10$^{13}$ cm$^{-2}$. A crossover from insulating phase to metallic state was clearly observed. The low-temperature charge transport mechanism is governed by two-dimensional (2D) variable-range hopping. This mechanism is influenced by band bending and gap states introduced by selenium vacancies. At low temperatures, the mobility is primarily limited by charged impurities, while at higher temperatures, it follows a power-law dependence, $μ= T^{-γ}$, indicating a dominance of electron-phonon scattering. The application of a gate field shifts the Fermi level toward the conduction band, and at sufficiently high temperatures, this drives the system into a metallic state. Our findings offer insights into the charge transport mechanisms in SnSe$_2$ FET, this understanding will allow for the optimization of other 2D materials for advanced electronic device applications.
title Metal-Insulator transition and Charge Transport Mechanisms in SnSe$_2$ Field-Effect Transistor
topic Materials Science
url https://arxiv.org/abs/2507.14536