Spatiotemporal organization of chemical oscillators via phase separation

Fuente: arXiv
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Main Authors: Bauermann, Jonathan, Bartolucci, Giacomo, Kolchinsky, Artemy
Format: Preprint
Published: 2025
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author Bauermann, Jonathan
Bartolucci, Giacomo
Kolchinsky, Artemy
author_facet Bauermann, Jonathan
Bartolucci, Giacomo
Kolchinsky, Artemy
contents We study chemical oscillators in the presence of phase separation. By imposing timescale separation between slow reactions and fast diffusion, we define a dynamics at phase equilibrium for the relevant degrees of freedom. We demonstrate that phase separation affects reaction kinetics by localizing reactants within phases, allowing for control of oscillator frequency and amplitude. The analysis is validated with a spatial model. Finally, relaxing the timescale separation between reactions and diffusion leads to waves of phase equilibria at mesoscopic scales.
format Preprint
id arxiv_https___arxiv_org_abs_2507_16030
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spatiotemporal organization of chemical oscillators via phase separation
Bauermann, Jonathan
Bartolucci, Giacomo
Kolchinsky, Artemy
Soft Condensed Matter
Pattern Formation and Solitons
Biological Physics
We study chemical oscillators in the presence of phase separation. By imposing timescale separation between slow reactions and fast diffusion, we define a dynamics at phase equilibrium for the relevant degrees of freedom. We demonstrate that phase separation affects reaction kinetics by localizing reactants within phases, allowing for control of oscillator frequency and amplitude. The analysis is validated with a spatial model. Finally, relaxing the timescale separation between reactions and diffusion leads to waves of phase equilibria at mesoscopic scales.
title Spatiotemporal organization of chemical oscillators via phase separation
topic Soft Condensed Matter
Pattern Formation and Solitons
Biological Physics
url https://arxiv.org/abs/2507.16030