Tuning chiral anomaly signature in a Dirac semimetal via fast-ion implantation

Fuente: arXiv
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Autores principales: Mandal, Manasi, Rha, Eunbi, Chotrattanapituk, Abhijatmedhi, Carrizales, Denisse Córdova, Lygo, Alexander, Woller, Kevin B., Cheng, Mouyang, Okabe, Ryotaro, Zhu, Guomin, Mak, Kiran, Fu, Chu-Liang, Liu, Chuhang, Wu, Lijun, Zhu, Yimei, Stemmer, Susanne, Li, Mingda
Formato: Preprint
Publicado: 2025
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author Mandal, Manasi
Rha, Eunbi
Chotrattanapituk, Abhijatmedhi
Carrizales, Denisse Córdova
Lygo, Alexander
Woller, Kevin B.
Cheng, Mouyang
Okabe, Ryotaro
Zhu, Guomin
Mak, Kiran
Fu, Chu-Liang
Liu, Chuhang
Wu, Lijun
Zhu, Yimei
Stemmer, Susanne
Li, Mingda
author_facet Mandal, Manasi
Rha, Eunbi
Chotrattanapituk, Abhijatmedhi
Carrizales, Denisse Córdova
Lygo, Alexander
Woller, Kevin B.
Cheng, Mouyang
Okabe, Ryotaro
Zhu, Guomin
Mak, Kiran
Fu, Chu-Liang
Liu, Chuhang
Wu, Lijun
Zhu, Yimei
Stemmer, Susanne
Li, Mingda
contents Cd$_3$As$_2$ is a prototypical Dirac semimetal that hosts a chiral anomaly and thereby functions as a platform to test high-energy physics hypotheses and to realize energy efficient applications. Here we use a combination of accelerator-based fast ion implantation and theory-driven planning to enhance the negative longitudinal magnetoresistance (NLMR)--a signature of a chiral anomaly--in Nb-doped Cd$_3$As$_2$ thin films. High-energy ion implantation is commonly used to investigate semiconductors and nuclear materials but is rarely employed to study quantum materials. We use electrical transport and transmission electron microscopy to characterize the NLMR and the crystallinity of Nb-doped Cd$_3$As$_2$ thin films. We find surface-doped Nb-Cd$_3$As$_2$ thin films display a maximum NLMR around $B = 7$ T and bulk-doped Nb-Cd$_3$As$_2$ thin films display a maximum NLMR over $B = 9$ T--all while maintaining crystallinity. This is more than a 100% relative enhancement of the maximum NLMR compared to pristine Cd$_3$As$_2$ thin films ($B = 4$ T). Our work demonstrates the potential of high-energy ion implantation as a practical route to realize chiralitronic functionalities in topological semimetals.
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institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Tuning chiral anomaly signature in a Dirac semimetal via fast-ion implantation
Mandal, Manasi
Rha, Eunbi
Chotrattanapituk, Abhijatmedhi
Carrizales, Denisse Córdova
Lygo, Alexander
Woller, Kevin B.
Cheng, Mouyang
Okabe, Ryotaro
Zhu, Guomin
Mak, Kiran
Fu, Chu-Liang
Liu, Chuhang
Wu, Lijun
Zhu, Yimei
Stemmer, Susanne
Li, Mingda
Materials Science
Cd$_3$As$_2$ is a prototypical Dirac semimetal that hosts a chiral anomaly and thereby functions as a platform to test high-energy physics hypotheses and to realize energy efficient applications. Here we use a combination of accelerator-based fast ion implantation and theory-driven planning to enhance the negative longitudinal magnetoresistance (NLMR)--a signature of a chiral anomaly--in Nb-doped Cd$_3$As$_2$ thin films. High-energy ion implantation is commonly used to investigate semiconductors and nuclear materials but is rarely employed to study quantum materials. We use electrical transport and transmission electron microscopy to characterize the NLMR and the crystallinity of Nb-doped Cd$_3$As$_2$ thin films. We find surface-doped Nb-Cd$_3$As$_2$ thin films display a maximum NLMR around $B = 7$ T and bulk-doped Nb-Cd$_3$As$_2$ thin films display a maximum NLMR over $B = 9$ T--all while maintaining crystallinity. This is more than a 100% relative enhancement of the maximum NLMR compared to pristine Cd$_3$As$_2$ thin films ($B = 4$ T). Our work demonstrates the potential of high-energy ion implantation as a practical route to realize chiralitronic functionalities in topological semimetals.
title Tuning chiral anomaly signature in a Dirac semimetal via fast-ion implantation
topic Materials Science
url https://arxiv.org/abs/2507.17972