Superconductivity from dual-surface carriers in rhombohedral graphene

Fuente: arXiv
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Hauptverfasser: Kumar, Manish, Waleffe, Derek, Okounkova, Anna, Tejani, Raveel, Phong, Vo Tien, Watanabe, Kenji, Taniguchi, Takashi, Lewandowski, Cyprian, Folk, Joshua, Yankowitz, Matthew
Format: Preprint
Veröffentlicht: 2025
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author Kumar, Manish
Waleffe, Derek
Okounkova, Anna
Tejani, Raveel
Phong, Vo Tien
Watanabe, Kenji
Taniguchi, Takashi
Lewandowski, Cyprian
Folk, Joshua
Yankowitz, Matthew
author_facet Kumar, Manish
Waleffe, Derek
Okounkova, Anna
Tejani, Raveel
Phong, Vo Tien
Watanabe, Kenji
Taniguchi, Takashi
Lewandowski, Cyprian
Folk, Joshua
Yankowitz, Matthew
contents Intrinsic rhombohedral graphene hosts an unusual low-energy electronic wavefunction, predominantly localized at its outer crystal faces with negligible presence in the bulk. Increasing the number of graphene layers amplifies the density of states near charge neutrality, greatly enhancing the susceptibility to symmetry-breaking phases. Here, we report superconductivity in rhombohedral graphene arising from an unusual charge-delocalized semimetallic normal state, characterized by coexisting valence- and conduction-band Fermi pockets split to opposite crystal surfaces. In octalayer graphene, the superconductivity appears in five apparently distinct pockets for each sign of an external electric displacement field ($D$). In a moiré superlattice sample where heptalayer graphene is aligned on one side to hexagonal boron nitride, two pockets of superconductivity emerge from a single sharp resistive feature. At higher $D$ the same resistive feature additionally induces an $h/e^{2}$-quantized anomalous Hall state at dopings near one electron per moiré unit cell. Our findings reveal a novel superconducting regime in multilayer graphene and create opportunities for coupling to nearby topological states.
format Preprint
id arxiv_https___arxiv_org_abs_2507_18598
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Superconductivity from dual-surface carriers in rhombohedral graphene
Kumar, Manish
Waleffe, Derek
Okounkova, Anna
Tejani, Raveel
Phong, Vo Tien
Watanabe, Kenji
Taniguchi, Takashi
Lewandowski, Cyprian
Folk, Joshua
Yankowitz, Matthew
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Superconductivity
Intrinsic rhombohedral graphene hosts an unusual low-energy electronic wavefunction, predominantly localized at its outer crystal faces with negligible presence in the bulk. Increasing the number of graphene layers amplifies the density of states near charge neutrality, greatly enhancing the susceptibility to symmetry-breaking phases. Here, we report superconductivity in rhombohedral graphene arising from an unusual charge-delocalized semimetallic normal state, characterized by coexisting valence- and conduction-band Fermi pockets split to opposite crystal surfaces. In octalayer graphene, the superconductivity appears in five apparently distinct pockets for each sign of an external electric displacement field ($D$). In a moiré superlattice sample where heptalayer graphene is aligned on one side to hexagonal boron nitride, two pockets of superconductivity emerge from a single sharp resistive feature. At higher $D$ the same resistive feature additionally induces an $h/e^{2}$-quantized anomalous Hall state at dopings near one electron per moiré unit cell. Our findings reveal a novel superconducting regime in multilayer graphene and create opportunities for coupling to nearby topological states.
title Superconductivity from dual-surface carriers in rhombohedral graphene
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2507.18598