A continuous-wave vacuum ultraviolet laser for the nuclear clock

Fuente: arXiv
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Auteurs principaux: Xiao, Qi, Penyazkov, Gleb, Li, Xiangliang, Huang, Beichen, Bu, Wenhao, Shi, Juanlang, Shi, Haoyu, Liao, Tangyin, Yan, Gaowei, Tian, Haochen, Li, Yixuan, Li, Jiatong, Lu, Bingkun, You, Li, Lin, Yige, Mo, Yuxiang, Ding, Shiqian
Format: Preprint
Publié: 2025
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author Xiao, Qi
Penyazkov, Gleb
Li, Xiangliang
Huang, Beichen
Bu, Wenhao
Shi, Juanlang
Shi, Haoyu
Liao, Tangyin
Yan, Gaowei
Tian, Haochen
Li, Yixuan
Li, Jiatong
Lu, Bingkun
You, Li
Lin, Yige
Mo, Yuxiang
Ding, Shiqian
author_facet Xiao, Qi
Penyazkov, Gleb
Li, Xiangliang
Huang, Beichen
Bu, Wenhao
Shi, Juanlang
Shi, Haoyu
Liao, Tangyin
Yan, Gaowei
Tian, Haochen
Li, Yixuan
Li, Jiatong
Lu, Bingkun
You, Li
Lin, Yige
Mo, Yuxiang
Ding, Shiqian
contents The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large ensembles of $^{229}$Th nuclei in transparent crystals and the development of pulsed vacuum-ultraviolet (VUV) lasers, have enabled initial laser spectroscopy of this transition. However, the lack of an intense, narrow-linewidth VUV laser has precluded coherent nuclear manipulation. Here we introduce and demonstrate the first continuous-wave laser at 148.4 nm, generated via four-wave mixing (FWM) in cadmium vapor. The source delivers 100 nW of power with a linewidth well below 100 Hz and supports broad wavelength tunability. This represents a five-orders-of-magnitude improvement in linewidth over all previous single-frequency lasers below 190 nm, marking a major advance in laser technology. We develop a spatially resolved homodyne technique to place a stringent upper bound on the phase noise induced by the FWM process and demonstrate sub-hertz linewidth capability. These results eliminate the final technical hurdle to a $^{229}$Th-based nuclear clock, opening new directions in quantum metrology, nuclear quantum optics and precision tests of the Standard Model. More broadly, they establish a widely tunable, ultranarrow-linewidth laser platform for applications across quantum information science, condensed matter physics, and high-resolution VUV spectroscopy.
format Preprint
id arxiv_https___arxiv_org_abs_2507_19449
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle A continuous-wave vacuum ultraviolet laser for the nuclear clock
Xiao, Qi
Penyazkov, Gleb
Li, Xiangliang
Huang, Beichen
Bu, Wenhao
Shi, Juanlang
Shi, Haoyu
Liao, Tangyin
Yan, Gaowei
Tian, Haochen
Li, Yixuan
Li, Jiatong
Lu, Bingkun
You, Li
Lin, Yige
Mo, Yuxiang
Ding, Shiqian
Atomic Physics
Optics
The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large ensembles of $^{229}$Th nuclei in transparent crystals and the development of pulsed vacuum-ultraviolet (VUV) lasers, have enabled initial laser spectroscopy of this transition. However, the lack of an intense, narrow-linewidth VUV laser has precluded coherent nuclear manipulation. Here we introduce and demonstrate the first continuous-wave laser at 148.4 nm, generated via four-wave mixing (FWM) in cadmium vapor. The source delivers 100 nW of power with a linewidth well below 100 Hz and supports broad wavelength tunability. This represents a five-orders-of-magnitude improvement in linewidth over all previous single-frequency lasers below 190 nm, marking a major advance in laser technology. We develop a spatially resolved homodyne technique to place a stringent upper bound on the phase noise induced by the FWM process and demonstrate sub-hertz linewidth capability. These results eliminate the final technical hurdle to a $^{229}$Th-based nuclear clock, opening new directions in quantum metrology, nuclear quantum optics and precision tests of the Standard Model. More broadly, they establish a widely tunable, ultranarrow-linewidth laser platform for applications across quantum information science, condensed matter physics, and high-resolution VUV spectroscopy.
title A continuous-wave vacuum ultraviolet laser for the nuclear clock
topic Atomic Physics
Optics
url https://arxiv.org/abs/2507.19449