Differentiation of Site-Specific Symmetry Breaking Orders in Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{6+y}$

Fuente: arXiv
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Hauptverfasser: Martinelli, L., Rüdiger, S., Bialo, I., Oppliger, J., Saldana, F. Igoa, Zimmermann, M. v., Weschke, E., Arpaia, R., Chang, J.
Format: Preprint
Veröffentlicht: 2025
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author Martinelli, L.
Rüdiger, S.
Bialo, I.
Oppliger, J.
Saldana, F. Igoa
Zimmermann, M. v.
Weschke, E.
Arpaia, R.
Chang, J.
author_facet Martinelli, L.
Rüdiger, S.
Bialo, I.
Oppliger, J.
Saldana, F. Igoa
Zimmermann, M. v.
Weschke, E.
Arpaia, R.
Chang, J.
contents Solid matter is classified through symmetry of ordering phenomena. Experimentally, this approach is straightforward, except when distinct orderings occur with identical or almost identical symmetry breaking. Here we show that the cuprate system Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{6+y}$ hosts two distinct orderings with almost identical translational symmetry breaking. Only when applying site-sensitive resonant elastic x-ray scattering (REXS), charge ordering can be conclusively differentiated from a super-lattice structure. These two orderings occur with almost the same in-plane symmetry but manifest at different atomic sites and display different temperature dependence. Differentiating these orders provides an important clue to the anomalous behavior of PrBa$_2$Cu$_3$O$_7$ within the 123-series of high-temperature superconductors. We conclude that the symmetry breaking at the Pr-site is unfavorable for superconducting pairing.
format Preprint
id arxiv_https___arxiv_org_abs_2507_20640
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Differentiation of Site-Specific Symmetry Breaking Orders in Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{6+y}$
Martinelli, L.
Rüdiger, S.
Bialo, I.
Oppliger, J.
Saldana, F. Igoa
Zimmermann, M. v.
Weschke, E.
Arpaia, R.
Chang, J.
Superconductivity
Strongly Correlated Electrons
Solid matter is classified through symmetry of ordering phenomena. Experimentally, this approach is straightforward, except when distinct orderings occur with identical or almost identical symmetry breaking. Here we show that the cuprate system Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{6+y}$ hosts two distinct orderings with almost identical translational symmetry breaking. Only when applying site-sensitive resonant elastic x-ray scattering (REXS), charge ordering can be conclusively differentiated from a super-lattice structure. These two orderings occur with almost the same in-plane symmetry but manifest at different atomic sites and display different temperature dependence. Differentiating these orders provides an important clue to the anomalous behavior of PrBa$_2$Cu$_3$O$_7$ within the 123-series of high-temperature superconductors. We conclude that the symmetry breaking at the Pr-site is unfavorable for superconducting pairing.
title Differentiation of Site-Specific Symmetry Breaking Orders in Y$_{1-x}$Pr$_x$Ba$_2$Cu$_3$O$_{6+y}$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2507.20640