Disorder driven crossover between anomalous Hall regimes in Fe$_3$GaTe$_2$

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Auteurs principaux: Lee, Sang-Eon, Park, Minkyu, Brown, W. Kice, Kulichenko, Vadym, Xin, Yan, Rhim, S. H., Hwang, Chanyong, Kim, Jaeyong, McCandless, Gregory T., Chan, Julia Y., Balicas, Luis
Format: Preprint
Publié: 2025
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author Lee, Sang-Eon
Park, Minkyu
Brown, W. Kice
Kulichenko, Vadym
Xin, Yan
Rhim, S. H.
Hwang, Chanyong
Kim, Jaeyong
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
author_facet Lee, Sang-Eon
Park, Minkyu
Brown, W. Kice
Kulichenko, Vadym
Xin, Yan
Rhim, S. H.
Hwang, Chanyong
Kim, Jaeyong
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
contents The large anomalous Hall conductivity (AHC) of the Fe$_3$(Ge,Ga)Te$_2$ compounds has attracted considerable attention. Here, we expose the intrinsic nature of AHC in Fe$_3$GaTe$_2$ crystals characterized by high conductivities, which show disorder-independent AHC with a pronounced value $σ_{xy}^{\text{c}}\approx$ 420 $Ω^{-1}$cm$^{-1}$. In the low conductivity regime, we observe the scaling relation $σ_{xy}\proptoσ_{xx}^{1.6}$, which crosses over to $σ_{xy} \simeq σ_{xy}^{\text{c}}$ as $σ_{xx}$ increases. Disorder in low-conductivity crystals is confirmed by the broadening of a first-order transition between ferromagnetism and the ferrimagnetic ground state. Through density functional theory (DFT) calculations, we reveal that the dominant sources of Berry curvature are located a few hundred meV below the Fermi energy around the $Γ$-point. Therefore, Fe$_3$GaTe$_2$ clearly exposes the disorder-induced crossover among distinct AHC regimes, previously inferred from measurements on different ferromagnets located in either side of the crossover region.
format Preprint
id arxiv_https___arxiv_org_abs_2507_23243
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Disorder driven crossover between anomalous Hall regimes in Fe$_3$GaTe$_2$
Lee, Sang-Eon
Park, Minkyu
Brown, W. Kice
Kulichenko, Vadym
Xin, Yan
Rhim, S. H.
Hwang, Chanyong
Kim, Jaeyong
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
Materials Science
The large anomalous Hall conductivity (AHC) of the Fe$_3$(Ge,Ga)Te$_2$ compounds has attracted considerable attention. Here, we expose the intrinsic nature of AHC in Fe$_3$GaTe$_2$ crystals characterized by high conductivities, which show disorder-independent AHC with a pronounced value $σ_{xy}^{\text{c}}\approx$ 420 $Ω^{-1}$cm$^{-1}$. In the low conductivity regime, we observe the scaling relation $σ_{xy}\proptoσ_{xx}^{1.6}$, which crosses over to $σ_{xy} \simeq σ_{xy}^{\text{c}}$ as $σ_{xx}$ increases. Disorder in low-conductivity crystals is confirmed by the broadening of a first-order transition between ferromagnetism and the ferrimagnetic ground state. Through density functional theory (DFT) calculations, we reveal that the dominant sources of Berry curvature are located a few hundred meV below the Fermi energy around the $Γ$-point. Therefore, Fe$_3$GaTe$_2$ clearly exposes the disorder-induced crossover among distinct AHC regimes, previously inferred from measurements on different ferromagnets located in either side of the crossover region.
title Disorder driven crossover between anomalous Hall regimes in Fe$_3$GaTe$_2$
topic Materials Science
url https://arxiv.org/abs/2507.23243