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Main Authors: Qin, Fanglu, Liu, Haiyang, Yang, Aosai, Liu, Yilin, Wang, Xuanji, Sun, Yue, Zhou, Xinyi, Sofer, Zdenek, Zhou, Jiayuan, Liu, Xue, Liu, Sheng, Zhang, Vanessa Li, Liu, Xiaoze, Gao, Weibo, Yu, Ting
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2508.00572
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author Qin, Fanglu
Liu, Haiyang
Yang, Aosai
Liu, Yilin
Wang, Xuanji
Sun, Yue
Zhou, Xinyi
Sofer, Zdenek
Zhou, Jiayuan
Liu, Xue
Liu, Sheng
Zhang, Vanessa Li
Liu, Xiaoze
Gao, Weibo
Yu, Ting
author_facet Qin, Fanglu
Liu, Haiyang
Yang, Aosai
Liu, Yilin
Wang, Xuanji
Sun, Yue
Zhou, Xinyi
Sofer, Zdenek
Zhou, Jiayuan
Liu, Xue
Liu, Sheng
Zhang, Vanessa Li
Liu, Xiaoze
Gao, Weibo
Yu, Ting
contents Emerging two-dimensional (2D) magnetic semiconductors represent transformative platforms to explore magneto-optics and opto-spintronic applications. Though 2D opto-spintronics has attracted tremendous research efforts in spin-dependent photodetectors and non-volatile memory components, the realization of one core application - spin-modulated light-emitting device (spin-LED) - remains elusive so far. Here we successfully realize prototype spin-LED integrated with a 2D semiconducting magnet CrSBr, demonstrating considerable electroluminescence (EL) down to bilayers. Intriguingly, the EL of the spin-LED is discovered to be directly manipulated by spin-flip and spin-canting transitions. Notably, spin-flip transitions enable unprecedented hysteretic behaviors of EL characteristics, while spin-canting transitions induce EL continuous modulation with robust anisotropy. This versatile manipulation is originated from the synergy of magnetic-order mediated excitonic transitions and spintronic transport. The prototype demonstration of spin-LED establishes an indispensable scheme of opto-spintronic devices leveraging 2D spin transitions and strong excitonic effects, presenting a critical step towards integrated 2D opto-spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2508_00572
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spin light-emitting devices in a 2D magnet
Qin, Fanglu
Liu, Haiyang
Yang, Aosai
Liu, Yilin
Wang, Xuanji
Sun, Yue
Zhou, Xinyi
Sofer, Zdenek
Zhou, Jiayuan
Liu, Xue
Liu, Sheng
Zhang, Vanessa Li
Liu, Xiaoze
Gao, Weibo
Yu, Ting
Applied Physics
Emerging two-dimensional (2D) magnetic semiconductors represent transformative platforms to explore magneto-optics and opto-spintronic applications. Though 2D opto-spintronics has attracted tremendous research efforts in spin-dependent photodetectors and non-volatile memory components, the realization of one core application - spin-modulated light-emitting device (spin-LED) - remains elusive so far. Here we successfully realize prototype spin-LED integrated with a 2D semiconducting magnet CrSBr, demonstrating considerable electroluminescence (EL) down to bilayers. Intriguingly, the EL of the spin-LED is discovered to be directly manipulated by spin-flip and spin-canting transitions. Notably, spin-flip transitions enable unprecedented hysteretic behaviors of EL characteristics, while spin-canting transitions induce EL continuous modulation with robust anisotropy. This versatile manipulation is originated from the synergy of magnetic-order mediated excitonic transitions and spintronic transport. The prototype demonstration of spin-LED establishes an indispensable scheme of opto-spintronic devices leveraging 2D spin transitions and strong excitonic effects, presenting a critical step towards integrated 2D opto-spintronics.
title Spin light-emitting devices in a 2D magnet
topic Applied Physics
url https://arxiv.org/abs/2508.00572