Enhanced spin-to-charge conversion in La$_{0.67}$Sr$_{0.33}$MnO$_3$/NdNiO$_3$ bilayers at the nickelate metal-insulator phase transition

Fuente: arXiv
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Main Authors: Sahoo, Biswajit, Das, Sarmistha, K, Akilan, Pofelski, Alexandre, Petit-Watelot, Sebastien, Rojas-Sánchez, Juan-Carlos, Zhu, Yimei, Frano, Alex, Fullerton, Eric E
Format: Preprint
Published: 2025
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author Sahoo, Biswajit
Das, Sarmistha
K, Akilan
Pofelski, Alexandre
Petit-Watelot, Sebastien
Rojas-Sánchez, Juan-Carlos
Zhu, Yimei
Frano, Alex
Fullerton, Eric E
author_facet Sahoo, Biswajit
Das, Sarmistha
K, Akilan
Pofelski, Alexandre
Petit-Watelot, Sebastien
Rojas-Sánchez, Juan-Carlos
Zhu, Yimei
Frano, Alex
Fullerton, Eric E
contents Phase transition materials such as NdNiO3 (NNO) when coupled with low damping ferromagnets such as La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) can lead to new multi-functional material systems harnessing the interplay of charge, spin and orbital degrees of freedom. In this study, we probe the evolution of the spin-to-charge conversion in epitaxial all-oxide LSMO (12 nm)/NNO (4, 8, and 16 nm) bilayers. Using spin pumping ferromagnetic resonance we track the spin-charge conversion in the NNO layer through the paramagnetic metal to antiferromagnetic insulator transition and observe a pronounced enhancement of the inverse spin Hall effect signal at the onset of this transition. We attribute this enhancement to the electronic and magnetic disorder in NNO at the first-order phase transition, thereby providing insights into the mechanism of spin transport through the phase transition. The tunability of spin charge conversion in this low damping bilayer system offers a pathway for developing multifunctional, energy-efficient spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2508_05300
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Enhanced spin-to-charge conversion in La$_{0.67}$Sr$_{0.33}$MnO$_3$/NdNiO$_3$ bilayers at the nickelate metal-insulator phase transition
Sahoo, Biswajit
Das, Sarmistha
K, Akilan
Pofelski, Alexandre
Petit-Watelot, Sebastien
Rojas-Sánchez, Juan-Carlos
Zhu, Yimei
Frano, Alex
Fullerton, Eric E
Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Phase transition materials such as NdNiO3 (NNO) when coupled with low damping ferromagnets such as La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) can lead to new multi-functional material systems harnessing the interplay of charge, spin and orbital degrees of freedom. In this study, we probe the evolution of the spin-to-charge conversion in epitaxial all-oxide LSMO (12 nm)/NNO (4, 8, and 16 nm) bilayers. Using spin pumping ferromagnetic resonance we track the spin-charge conversion in the NNO layer through the paramagnetic metal to antiferromagnetic insulator transition and observe a pronounced enhancement of the inverse spin Hall effect signal at the onset of this transition. We attribute this enhancement to the electronic and magnetic disorder in NNO at the first-order phase transition, thereby providing insights into the mechanism of spin transport through the phase transition. The tunability of spin charge conversion in this low damping bilayer system offers a pathway for developing multifunctional, energy-efficient spintronic devices.
title Enhanced spin-to-charge conversion in La$_{0.67}$Sr$_{0.33}$MnO$_3$/NdNiO$_3$ bilayers at the nickelate metal-insulator phase transition
topic Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2508.05300