High-definition 3D suspended Archimedean spiral with broadband, spatially extended, and single-handed optical chirality enhancement in Vis-NIR range

Fuente: arXiv
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Autores principales: Jiang, Min, Chakraborty, Abhik, Wu, Xiaofei, Tan, Hark Hoe, Huang, Jer-Shing
Formato: Preprint
Publicado: 2025
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author Jiang, Min
Chakraborty, Abhik
Wu, Xiaofei
Tan, Hark Hoe
Huang, Jer-Shing
author_facet Jiang, Min
Chakraborty, Abhik
Wu, Xiaofei
Tan, Hark Hoe
Huang, Jer-Shing
contents 3D plasmonic structures can provide giant optical chirality (C) in the near field, enabling strong interactions with enantiomers for chiral sensing applications. However, these structures face several limitations, including narrow operational bandwidth constrained by resonance, flipping handedness of C around the resonant frequency, spatially confined distribution of C, and difficulty in trapping enantiomers. Our numerical predictions reveal that a 3D plasmonic Archimedean spiral (AS) exhibits spectrally broadband, spatially extended and single-handed near-field C in visible-to-near-infrared range. However, realizing highly deterministic 3D AS remains challenging. We develop an effective fabrication strategy that combines focused ion beam milling and template-stripping method to realize high-definition 3D AS. Furthermore, we experimentally characterize the fabricated structure's far-field chiroptical behavior to confirm the predicted optical response. Owing to its conical hole-like geometry, 3D AS can potentially function as a sieve for trapping enantiomer-functionalized nanoparticles in the hot zone with enhanced C for sensitive broadband chirotical detection.
format Preprint
id arxiv_https___arxiv_org_abs_2508_09433
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle High-definition 3D suspended Archimedean spiral with broadband, spatially extended, and single-handed optical chirality enhancement in Vis-NIR range
Jiang, Min
Chakraborty, Abhik
Wu, Xiaofei
Tan, Hark Hoe
Huang, Jer-Shing
Optics
78A70
J.2
3D plasmonic structures can provide giant optical chirality (C) in the near field, enabling strong interactions with enantiomers for chiral sensing applications. However, these structures face several limitations, including narrow operational bandwidth constrained by resonance, flipping handedness of C around the resonant frequency, spatially confined distribution of C, and difficulty in trapping enantiomers. Our numerical predictions reveal that a 3D plasmonic Archimedean spiral (AS) exhibits spectrally broadband, spatially extended and single-handed near-field C in visible-to-near-infrared range. However, realizing highly deterministic 3D AS remains challenging. We develop an effective fabrication strategy that combines focused ion beam milling and template-stripping method to realize high-definition 3D AS. Furthermore, we experimentally characterize the fabricated structure's far-field chiroptical behavior to confirm the predicted optical response. Owing to its conical hole-like geometry, 3D AS can potentially function as a sieve for trapping enantiomer-functionalized nanoparticles in the hot zone with enhanced C for sensitive broadband chirotical detection.
title High-definition 3D suspended Archimedean spiral with broadband, spatially extended, and single-handed optical chirality enhancement in Vis-NIR range
topic Optics
78A70
J.2
url https://arxiv.org/abs/2508.09433