Emergent Interacting Phases in the Strong Coupling Limit of Twisted M-Valley Moiré Systems: Application to SnSe${}_2$

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Auteurs principaux: Li, Ming-Rui, Calugaru, Dumitru, Jiang, Yi, Pi, Hanqi, Fischer, Ammon, Schlömer, Henning, Klebl, Lennart, Vergniory, Maia G., Kennes, Dante M., Parameswaran, Siddharth A., Yao, Hong, Bernevig, B. Andrei, Hu, Haoyu
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Publié: 2025
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author Li, Ming-Rui
Calugaru, Dumitru
Jiang, Yi
Pi, Hanqi
Fischer, Ammon
Schlömer, Henning
Klebl, Lennart
Vergniory, Maia G.
Kennes, Dante M.
Parameswaran, Siddharth A.
Yao, Hong
Bernevig, B. Andrei
Hu, Haoyu
author_facet Li, Ming-Rui
Calugaru, Dumitru
Jiang, Yi
Pi, Hanqi
Fischer, Ammon
Schlömer, Henning
Klebl, Lennart
Vergniory, Maia G.
Kennes, Dante M.
Parameswaran, Siddharth A.
Yao, Hong
Bernevig, B. Andrei
Hu, Haoyu
contents We construct an interacting Wannier model for both AA-stacked and AB-stacked twisted SnSe2, revealing a rich landscape of correlated quantum phases. For the AA-stacked case, the system is effectively described by a three-orbital triangular lattice model, where each orbital corresponds to a valley and exhibits an approximate one-dimensional hopping structure due to a new momentum-space non-symmorphic symmetry. By exploring the interacting phase diagram using a combination of theoretical methods, including Hartree-Fock mean-field theory and exact solutions of the spin model in certain limits, we identify several exotic quantum phases. These include a dimerized phase with finite residual entropy, valence bond solids, and quantum paramagnetism. In the AB-stacked case, the system realizes an interacting kagome lattice model, where the Wannier orbitals associated with the three valleys form three sublattices. In the strong coupling regime, we use cluster mean-field methods to demonstrate the emergence of a classical spin liquid phase due to the frustrated lattice structure. The high tunability of the moiré system, which allows control over both the filling and interaction strength (via twist angle), renders twisted SnSe2 a versatile platform for realizing a wide range of exotic correlated quantum phases.
format Preprint
id arxiv_https___arxiv_org_abs_2508_10098
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Emergent Interacting Phases in the Strong Coupling Limit of Twisted M-Valley Moiré Systems: Application to SnSe${}_2$
Li, Ming-Rui
Calugaru, Dumitru
Jiang, Yi
Pi, Hanqi
Fischer, Ammon
Schlömer, Henning
Klebl, Lennart
Vergniory, Maia G.
Kennes, Dante M.
Parameswaran, Siddharth A.
Yao, Hong
Bernevig, B. Andrei
Hu, Haoyu
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
We construct an interacting Wannier model for both AA-stacked and AB-stacked twisted SnSe2, revealing a rich landscape of correlated quantum phases. For the AA-stacked case, the system is effectively described by a three-orbital triangular lattice model, where each orbital corresponds to a valley and exhibits an approximate one-dimensional hopping structure due to a new momentum-space non-symmorphic symmetry. By exploring the interacting phase diagram using a combination of theoretical methods, including Hartree-Fock mean-field theory and exact solutions of the spin model in certain limits, we identify several exotic quantum phases. These include a dimerized phase with finite residual entropy, valence bond solids, and quantum paramagnetism. In the AB-stacked case, the system realizes an interacting kagome lattice model, where the Wannier orbitals associated with the three valleys form three sublattices. In the strong coupling regime, we use cluster mean-field methods to demonstrate the emergence of a classical spin liquid phase due to the frustrated lattice structure. The high tunability of the moiré system, which allows control over both the filling and interaction strength (via twist angle), renders twisted SnSe2 a versatile platform for realizing a wide range of exotic correlated quantum phases.
title Emergent Interacting Phases in the Strong Coupling Limit of Twisted M-Valley Moiré Systems: Application to SnSe${}_2$
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2508.10098