Fast hydrogen atom diffraction through monocrystalline graphene

Fuente: arXiv
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Main Authors: Guichard, Pierre, Dochain, Arnaud, Marion, Raphaël, de Picquendaele, Pauline de Crombrugghe, Lejeune, Nicolas, Hackens, Benoît, Hervieux, Paul-Antoine, Urbain, Xavier
Format: Preprint
Published: 2025
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author Guichard, Pierre
Dochain, Arnaud
Marion, Raphaël
de Picquendaele, Pauline de Crombrugghe
Lejeune, Nicolas
Hackens, Benoît
Hervieux, Paul-Antoine
Urbain, Xavier
author_facet Guichard, Pierre
Dochain, Arnaud
Marion, Raphaël
de Picquendaele, Pauline de Crombrugghe
Lejeune, Nicolas
Hackens, Benoît
Hervieux, Paul-Antoine
Urbain, Xavier
contents We report fast atom diffraction through single-layer graphene using hydrogen atoms at kinetic energies from 150 to 1200 eV. High-resolution images reveal overlapping hexagonal patterns from coexisting monocrystalline domains. Time-of-flight tagging confirms negligible energy loss, making the method suitable for matter-wave interferometry. The diffraction is well described by the eikonal approximation, with accurate modeling requiring the full 3D interaction potential from DFT. Simpler models fail to reproduce the data, highlighting the exceptional sensitivity of diffraction patterns to atom-surface interactions and their potential for spectroscopic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2508_13175
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Fast hydrogen atom diffraction through monocrystalline graphene
Guichard, Pierre
Dochain, Arnaud
Marion, Raphaël
de Picquendaele, Pauline de Crombrugghe
Lejeune, Nicolas
Hackens, Benoît
Hervieux, Paul-Antoine
Urbain, Xavier
Mesoscale and Nanoscale Physics
Atomic Physics
Quantum Physics
We report fast atom diffraction through single-layer graphene using hydrogen atoms at kinetic energies from 150 to 1200 eV. High-resolution images reveal overlapping hexagonal patterns from coexisting monocrystalline domains. Time-of-flight tagging confirms negligible energy loss, making the method suitable for matter-wave interferometry. The diffraction is well described by the eikonal approximation, with accurate modeling requiring the full 3D interaction potential from DFT. Simpler models fail to reproduce the data, highlighting the exceptional sensitivity of diffraction patterns to atom-surface interactions and their potential for spectroscopic applications.
title Fast hydrogen atom diffraction through monocrystalline graphene
topic Mesoscale and Nanoscale Physics
Atomic Physics
Quantum Physics
url https://arxiv.org/abs/2508.13175