Production of ultracold asymmetric tops from Sr atoms and SrOH molecules

Fuente: arXiv
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Autori principali: Kosicki, Maciej B., Borkowski, Mateusz, Umiński, Marcin, Żuchowski, Piotr S.
Natura: Preprint
Pubblicazione: 2025
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author Kosicki, Maciej B.
Borkowski, Mateusz
Umiński, Marcin
Żuchowski, Piotr S.
author_facet Kosicki, Maciej B.
Borkowski, Mateusz
Umiński, Marcin
Żuchowski, Piotr S.
contents We report the comprehensive theoretical investigation of the Sr-SrOH system identifying it as a promising route to production of ultracold asymmetric top molecules. Combining high-level ab initio electronic structure calculations with rigorous quantum scattering simulations, we determine strongly anisotropic, non-reactive interaction potential and an exceptionally dense spectrum of near-threshold resonances. Presented excited states, transition dipole moments, and results of the one-dimensional STIRAP model suggest the possibility of coherently transferring weakly bound complexes to the rovibrational ground state.
format Preprint
id arxiv_https___arxiv_org_abs_2508_14543
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Production of ultracold asymmetric tops from Sr atoms and SrOH molecules
Kosicki, Maciej B.
Borkowski, Mateusz
Umiński, Marcin
Żuchowski, Piotr S.
Atomic Physics
Quantum Gases
Chemical Physics
We report the comprehensive theoretical investigation of the Sr-SrOH system identifying it as a promising route to production of ultracold asymmetric top molecules. Combining high-level ab initio electronic structure calculations with rigorous quantum scattering simulations, we determine strongly anisotropic, non-reactive interaction potential and an exceptionally dense spectrum of near-threshold resonances. Presented excited states, transition dipole moments, and results of the one-dimensional STIRAP model suggest the possibility of coherently transferring weakly bound complexes to the rovibrational ground state.
title Production of ultracold asymmetric tops from Sr atoms and SrOH molecules
topic Atomic Physics
Quantum Gases
Chemical Physics
url https://arxiv.org/abs/2508.14543