Superconductivity and Ferroelectric Orbital Magnetism in Semimetallic Rhombohedral Hexalayer Graphene

Fuente: arXiv
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Auteurs principaux: Deng, Jinghao, Xie, Jiabin, Li, Hongyuan, Taniguchi, Takashi, Watanabe, Kenji, Shan, Jie, Mak, Kin Fai, Liu, Xiaomeng
Format: Preprint
Publié: 2025
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author Deng, Jinghao
Xie, Jiabin
Li, Hongyuan
Taniguchi, Takashi
Watanabe, Kenji
Shan, Jie
Mak, Kin Fai
Liu, Xiaomeng
author_facet Deng, Jinghao
Xie, Jiabin
Li, Hongyuan
Taniguchi, Takashi
Watanabe, Kenji
Shan, Jie
Mak, Kin Fai
Liu, Xiaomeng
contents Rhombohedral multilayer graphene has emerged as a promising platform for exploring correlated and topological quantum phases, enabled by its Berry-curvature-bearing flat bands. While prior work has focused on separated conduction and valence bands, we probe the extensive semimetallic regime of rhombohedral hexalayer graphene. We survey a rich phase diagram dominated by flavor-symmetry breaking and reveal an electric-field-driven band inversion by fermiology. Near this inversion, we observe two superconducting-like states confined to regions with coexisting electron and hole Fermi surfaces, suggesting a possible dual-carrier origin. In addition, we identify a ferroelectric orbital magnet that undergoes sharp switching under unipolar electric fields, signaling spontaneous electric polarization. Unlike previously reported multiferroicity near zero electric field, this new state exhibits magnetic hysteresis reversible by electric field, consistent with a phenomenological model of coupled electric and magnetic polarization. Our work elucidates the correlated semimetal regime in rhombohedral graphene and underscores its potential to host diverse quantum phases.
format Preprint
id arxiv_https___arxiv_org_abs_2508_15909
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Superconductivity and Ferroelectric Orbital Magnetism in Semimetallic Rhombohedral Hexalayer Graphene
Deng, Jinghao
Xie, Jiabin
Li, Hongyuan
Taniguchi, Takashi
Watanabe, Kenji
Shan, Jie
Mak, Kin Fai
Liu, Xiaomeng
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Rhombohedral multilayer graphene has emerged as a promising platform for exploring correlated and topological quantum phases, enabled by its Berry-curvature-bearing flat bands. While prior work has focused on separated conduction and valence bands, we probe the extensive semimetallic regime of rhombohedral hexalayer graphene. We survey a rich phase diagram dominated by flavor-symmetry breaking and reveal an electric-field-driven band inversion by fermiology. Near this inversion, we observe two superconducting-like states confined to regions with coexisting electron and hole Fermi surfaces, suggesting a possible dual-carrier origin. In addition, we identify a ferroelectric orbital magnet that undergoes sharp switching under unipolar electric fields, signaling spontaneous electric polarization. Unlike previously reported multiferroicity near zero electric field, this new state exhibits magnetic hysteresis reversible by electric field, consistent with a phenomenological model of coupled electric and magnetic polarization. Our work elucidates the correlated semimetal regime in rhombohedral graphene and underscores its potential to host diverse quantum phases.
title Superconductivity and Ferroelectric Orbital Magnetism in Semimetallic Rhombohedral Hexalayer Graphene
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2508.15909