Studying the effect of the phonon coherence and inflow on the formation of hydrogen bonds in the $[(\rm{H}_2\rm{O})_2]^m$ cluster

Fuente: arXiv
Salvato in:
Dettagli Bibliografici
Autore principale: Miao, Hui-hui
Natura: Preprint
Pubblicazione: 2025
Soggetti:
Accesso online:
Tags: Aggiungi Tag
Nessun Tag, puoi essere il primo ad aggiungerne!!
_version_ 1866915460180606976
author Miao, Hui-hui
author_facet Miao, Hui-hui
contents In this paper, a simple $\rm{H}_2\rm{O}$-related hydrogen-bonded model is proposed, and different types of phonons are introduced to describe the macro- and micro- vibrations of particles in this model. $[(\rm{H}_2\rm{O})_2]^m$ cluster consisting of hydrogen-bonded systems is considered. The effect of phonon coherence on both unitary and dissipative evolutions is studied and compared with the incoherent case. Consideration is given to the dark states -- coherent states that arise from the evolution of open quantum systems. Consideration is also given to the effect of all potential phonon inflows on evolution. The results reveal important effects of phonon coherence and inflow on the dynamics of clusters and will be used as a basis to extend the research to more complex chemical and biological models.
format Preprint
id arxiv_https___arxiv_org_abs_2508_17089
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Studying the effect of the phonon coherence and inflow on the formation of hydrogen bonds in the $[(\rm{H}_2\rm{O})_2]^m$ cluster
Miao, Hui-hui
Quantum Physics
In this paper, a simple $\rm{H}_2\rm{O}$-related hydrogen-bonded model is proposed, and different types of phonons are introduced to describe the macro- and micro- vibrations of particles in this model. $[(\rm{H}_2\rm{O})_2]^m$ cluster consisting of hydrogen-bonded systems is considered. The effect of phonon coherence on both unitary and dissipative evolutions is studied and compared with the incoherent case. Consideration is given to the dark states -- coherent states that arise from the evolution of open quantum systems. Consideration is also given to the effect of all potential phonon inflows on evolution. The results reveal important effects of phonon coherence and inflow on the dynamics of clusters and will be used as a basis to extend the research to more complex chemical and biological models.
title Studying the effect of the phonon coherence and inflow on the formation of hydrogen bonds in the $[(\rm{H}_2\rm{O})_2]^m$ cluster
topic Quantum Physics
url https://arxiv.org/abs/2508.17089