Role of interlayer shear phonons on lattice symmetry switching in the transition metal dichalcogenide WTe$_{2}$

Fuente: arXiv
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Main Authors: Akei, Mizuki, Fukuda, Takumi, Mizukoshi, Yu, Kikuchi, Kazuhiro, Hase, Muneaki
Format: Preprint
Published: 2025
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author Akei, Mizuki
Fukuda, Takumi
Mizukoshi, Yu
Kikuchi, Kazuhiro
Hase, Muneaki
author_facet Akei, Mizuki
Fukuda, Takumi
Mizukoshi, Yu
Kikuchi, Kazuhiro
Hase, Muneaki
contents Coherent phonon control using ultrashort pulse trains is the key to realizing structural phase transitions in solids by non-thermal pathways. By combining double-pulse excitation and time-resolved second harmonic generation techniques under high-density electronic excitation in a 2D layered material, WTe$_{2}$, we demonstrate that the lattice symmetry switching from the Weyl semimetallic T$_{d}$ to the semimetallic 1T$^{\prime}$ phases is independent of the amplitude of the coherent interlayer shear phonons after the arrival of the second pump pulse. This finding provides new insights into the mechanisms for symmetry switching that electronic excitation-driven shear sliding plays a dominant role.
format Preprint
id arxiv_https___arxiv_org_abs_2508_17939
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Role of interlayer shear phonons on lattice symmetry switching in the transition metal dichalcogenide WTe$_{2}$
Akei, Mizuki
Fukuda, Takumi
Mizukoshi, Yu
Kikuchi, Kazuhiro
Hase, Muneaki
Materials Science
Coherent phonon control using ultrashort pulse trains is the key to realizing structural phase transitions in solids by non-thermal pathways. By combining double-pulse excitation and time-resolved second harmonic generation techniques under high-density electronic excitation in a 2D layered material, WTe$_{2}$, we demonstrate that the lattice symmetry switching from the Weyl semimetallic T$_{d}$ to the semimetallic 1T$^{\prime}$ phases is independent of the amplitude of the coherent interlayer shear phonons after the arrival of the second pump pulse. This finding provides new insights into the mechanisms for symmetry switching that electronic excitation-driven shear sliding plays a dominant role.
title Role of interlayer shear phonons on lattice symmetry switching in the transition metal dichalcogenide WTe$_{2}$
topic Materials Science
url https://arxiv.org/abs/2508.17939