Study of low-energy electron-induced dissociation of 1-Propanol

Fuente: arXiv
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Main Authors: Ghosh, Soumya, Chakraborty, Dipayan, Paul, Anirban, Nandi, Dhananjay
Format: Preprint
Published: 2025
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_version_ 1866910012514762752
author Ghosh, Soumya
Chakraborty, Dipayan
Paul, Anirban
Nandi, Dhananjay
author_facet Ghosh, Soumya
Chakraborty, Dipayan
Paul, Anirban
Nandi, Dhananjay
contents The fragmentation of 1-propanol resulting from dissociative electron attachment has been explored across an energy range of 3.5 to 16 eV. Four distinct ion species are identified: $\text{H}^{-}$, $\text{O}^{-}$, $\text{OH}^{-}$, and $\text{C}_{3}\text{H}_{7}\text{O}^{-}$. The $\text{OH}^{-}$ ion exhibited a prominent peak near 8.7 eV, along with a small hump near 5.6 eV. Complementary channels led to the formation of the $\text{H}^{-}$ and $\text{C}_{3}\text{H}_{7}\text{O}^{-}$ ions. Both these two ions exhibit a sharp peak near 6 eV and broad overlapping resonances between 7 to 12 eV. The observed ion yields of distinct dissociation fragments in this study, when compared with those from previously studied alcohols, suggest site-specific fragmentation of alcohols during dissociative electron attachment. To gain a deeper understanding of the dissociation pathways, Density Functional Theory~(DFT) calculations were conducted, revealing the threshold energies for each channel. These threshold energies aligned well with the experimental uncertainties.
format Preprint
id arxiv_https___arxiv_org_abs_2508_19685
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Study of low-energy electron-induced dissociation of 1-Propanol
Ghosh, Soumya
Chakraborty, Dipayan
Paul, Anirban
Nandi, Dhananjay
Atomic and Molecular Clusters
Atomic Physics
Chemical Physics
The fragmentation of 1-propanol resulting from dissociative electron attachment has been explored across an energy range of 3.5 to 16 eV. Four distinct ion species are identified: $\text{H}^{-}$, $\text{O}^{-}$, $\text{OH}^{-}$, and $\text{C}_{3}\text{H}_{7}\text{O}^{-}$. The $\text{OH}^{-}$ ion exhibited a prominent peak near 8.7 eV, along with a small hump near 5.6 eV. Complementary channels led to the formation of the $\text{H}^{-}$ and $\text{C}_{3}\text{H}_{7}\text{O}^{-}$ ions. Both these two ions exhibit a sharp peak near 6 eV and broad overlapping resonances between 7 to 12 eV. The observed ion yields of distinct dissociation fragments in this study, when compared with those from previously studied alcohols, suggest site-specific fragmentation of alcohols during dissociative electron attachment. To gain a deeper understanding of the dissociation pathways, Density Functional Theory~(DFT) calculations were conducted, revealing the threshold energies for each channel. These threshold energies aligned well with the experimental uncertainties.
title Study of low-energy electron-induced dissociation of 1-Propanol
topic Atomic and Molecular Clusters
Atomic Physics
Chemical Physics
url https://arxiv.org/abs/2508.19685