Magnetic resonance and microwave resistance modulation in van der Waals colossal-magnetoresistance material

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Hauptverfasser: Tanaka, Miuko, Ahad, Abdul, Deaconu, Darius-Alexandru, Shah, Varun, Nishio-Hamane, Daisuke, Ishii, Tomohiro, Hashisaka, Masayuki, Sakamoto, Shoya, Miwa, Shinji, Bahramy, Mohammad Saeed, Ideue, Toshiya
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Veröffentlicht: 2025
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author Tanaka, Miuko
Ahad, Abdul
Deaconu, Darius-Alexandru
Shah, Varun
Nishio-Hamane, Daisuke
Ishii, Tomohiro
Hashisaka, Masayuki
Sakamoto, Shoya
Miwa, Shinji
Bahramy, Mohammad Saeed
Ideue, Toshiya
author_facet Tanaka, Miuko
Ahad, Abdul
Deaconu, Darius-Alexandru
Shah, Varun
Nishio-Hamane, Daisuke
Ishii, Tomohiro
Hashisaka, Masayuki
Sakamoto, Shoya
Miwa, Shinji
Bahramy, Mohammad Saeed
Ideue, Toshiya
contents Colossal magnetoresistance (CMR) is a fascinating quantum phenomenon that continues to draw significant interest in condensed matter physics. Mn3Si2Te6 has emerged as a prototypical CMR material, notable for its puzzling magnetoresistance behavior and pronounced directional anisotropy. Despite extensive research, the mechanisms driving CMR in Mn3Si2Te6 remain elusive [1-4]. In this work, we explore the magnetic resonance of Mn3Si2Te6 and observe a reduced g-factor for magnetic fields applied along the crystalline c-axis compared to the ab-plane, indicating a substantial orbital magnetization contribution along the c-axis. Furthermore, we detect resistance modulation under resonance conditions, suggesting that CMR in Mn3Si2Te6 is sensitive to the out-of-the plane spin polarization. These findings shed new light on the role of orbital magnetic moment in Mn3Si2Te6, offering a deeper understanding of the interplay between spin, orbital and lattice degrees of freedom of electrons in this system.
format Preprint
id arxiv_https___arxiv_org_abs_2509_02901
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Magnetic resonance and microwave resistance modulation in van der Waals colossal-magnetoresistance material
Tanaka, Miuko
Ahad, Abdul
Deaconu, Darius-Alexandru
Shah, Varun
Nishio-Hamane, Daisuke
Ishii, Tomohiro
Hashisaka, Masayuki
Sakamoto, Shoya
Miwa, Shinji
Bahramy, Mohammad Saeed
Ideue, Toshiya
Materials Science
Mesoscale and Nanoscale Physics
Colossal magnetoresistance (CMR) is a fascinating quantum phenomenon that continues to draw significant interest in condensed matter physics. Mn3Si2Te6 has emerged as a prototypical CMR material, notable for its puzzling magnetoresistance behavior and pronounced directional anisotropy. Despite extensive research, the mechanisms driving CMR in Mn3Si2Te6 remain elusive [1-4]. In this work, we explore the magnetic resonance of Mn3Si2Te6 and observe a reduced g-factor for magnetic fields applied along the crystalline c-axis compared to the ab-plane, indicating a substantial orbital magnetization contribution along the c-axis. Furthermore, we detect resistance modulation under resonance conditions, suggesting that CMR in Mn3Si2Te6 is sensitive to the out-of-the plane spin polarization. These findings shed new light on the role of orbital magnetic moment in Mn3Si2Te6, offering a deeper understanding of the interplay between spin, orbital and lattice degrees of freedom of electrons in this system.
title Magnetic resonance and microwave resistance modulation in van der Waals colossal-magnetoresistance material
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2509.02901