Octupole-driven spin-transfer torque switching of all-antiferromagnetic tunnel junctions

Fuente: arXiv
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Auteurs principaux: Kang, Jaimin, Hamdi, Mohammad, Cheung, Shun Kong, Yuan, Lin-Ding, Elekhtiar, Mohamed, Rogers, William, Meo, Andrea, Lim, Peter G., Tey, M. S. Nicholas, D'Addario, Anthony, Konakanchi, Shiva T., Matt, Eric, Athas, Jordan, Arpaci, Sevdenur, Wan, Lei, Mehta, Sanjay C., Upadhyaya, Pramey, Carpentieri, Mario, Dravid, Vinayak P., Hersam, Mark C., Katine, Jordan A., Fuchs, Gregory D., Finocchio, Giovanni, Tsymbal, Evgeny Y., Rondinelli, James M., Amiri, Pedram Khalili
Format: Preprint
Publié: 2025
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author Kang, Jaimin
Hamdi, Mohammad
Cheung, Shun Kong
Yuan, Lin-Ding
Elekhtiar, Mohamed
Rogers, William
Meo, Andrea
Lim, Peter G.
Tey, M. S. Nicholas
D'Addario, Anthony
Konakanchi, Shiva T.
Matt, Eric
Athas, Jordan
Arpaci, Sevdenur
Wan, Lei
Mehta, Sanjay C.
Upadhyaya, Pramey
Carpentieri, Mario
Dravid, Vinayak P.
Hersam, Mark C.
Katine, Jordan A.
Fuchs, Gregory D.
Finocchio, Giovanni
Tsymbal, Evgeny Y.
Rondinelli, James M.
Amiri, Pedram Khalili
author_facet Kang, Jaimin
Hamdi, Mohammad
Cheung, Shun Kong
Yuan, Lin-Ding
Elekhtiar, Mohamed
Rogers, William
Meo, Andrea
Lim, Peter G.
Tey, M. S. Nicholas
D'Addario, Anthony
Konakanchi, Shiva T.
Matt, Eric
Athas, Jordan
Arpaci, Sevdenur
Wan, Lei
Mehta, Sanjay C.
Upadhyaya, Pramey
Carpentieri, Mario
Dravid, Vinayak P.
Hersam, Mark C.
Katine, Jordan A.
Fuchs, Gregory D.
Finocchio, Giovanni
Tsymbal, Evgeny Y.
Rondinelli, James M.
Amiri, Pedram Khalili
contents Magnetic tunnel junctions (MTJs) based on ferromagnets are canonical devices in spintronics, with wide-ranging applications in data storage, computing, and sensing. They simultaneously exhibit mechanisms for electrical detection of magnetic order through the tunneling magnetoresistance (TMR) effect, and reciprocally, for controlling magnetic order by electric currents through spin-transfer torque (STT). It was long assumed that neither of these effects could be sizeable in tunnel junctions made from antiferromagnetic materials, since they exhibit no net magnetization. Recently, however, it was shown that all-antiferromagnetic tunnel junctions (AFMTJs) based on chiral antiferromagnets do exhibit TMR due to their non-relativistic momentum-dependent spin polarization and cluster magnetic octupole moment, which are manifestations of their spin-split band structure. However, the reciprocal effect, i.e., the antiferromagnetic counterpart of STT driven by currents through the AFMTJ, has been assumed non-existent due to the total electric current being spin-neutral. Here, in contrast to this common expectation, we report nanoscale AFMTJs exhibiting this reciprocal effect, which we term octupole-driven spin-transfer torque (OTT). We demonstrate current-induced OTT switching of PtMn3|MgO|PtMn3 AFMTJs, fabricated on a thermally oxidized silicon substrate, exhibiting a record-high TMR value of 363% at room temperature and switching current densities of the order of 10 MA/cm2. Our theoretical modeling explains the origin of OTT in terms of the imbalance between intra- and inter-sublattice spin currents across the AFMTJ, and equivalently, in terms of the non-zero net cluster octupole polarization of each PtMn3 layer. This work establishes a new materials platform for antiferromagnetic spintronics and provides a pathway towards deeply scaled magnetic memory and room-temperature terahertz technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2509_03026
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Octupole-driven spin-transfer torque switching of all-antiferromagnetic tunnel junctions
Kang, Jaimin
Hamdi, Mohammad
Cheung, Shun Kong
Yuan, Lin-Ding
Elekhtiar, Mohamed
Rogers, William
Meo, Andrea
Lim, Peter G.
Tey, M. S. Nicholas
D'Addario, Anthony
Konakanchi, Shiva T.
Matt, Eric
Athas, Jordan
Arpaci, Sevdenur
Wan, Lei
Mehta, Sanjay C.
Upadhyaya, Pramey
Carpentieri, Mario
Dravid, Vinayak P.
Hersam, Mark C.
Katine, Jordan A.
Fuchs, Gregory D.
Finocchio, Giovanni
Tsymbal, Evgeny Y.
Rondinelli, James M.
Amiri, Pedram Khalili
Materials Science
Mesoscale and Nanoscale Physics
Applied Physics
Magnetic tunnel junctions (MTJs) based on ferromagnets are canonical devices in spintronics, with wide-ranging applications in data storage, computing, and sensing. They simultaneously exhibit mechanisms for electrical detection of magnetic order through the tunneling magnetoresistance (TMR) effect, and reciprocally, for controlling magnetic order by electric currents through spin-transfer torque (STT). It was long assumed that neither of these effects could be sizeable in tunnel junctions made from antiferromagnetic materials, since they exhibit no net magnetization. Recently, however, it was shown that all-antiferromagnetic tunnel junctions (AFMTJs) based on chiral antiferromagnets do exhibit TMR due to their non-relativistic momentum-dependent spin polarization and cluster magnetic octupole moment, which are manifestations of their spin-split band structure. However, the reciprocal effect, i.e., the antiferromagnetic counterpart of STT driven by currents through the AFMTJ, has been assumed non-existent due to the total electric current being spin-neutral. Here, in contrast to this common expectation, we report nanoscale AFMTJs exhibiting this reciprocal effect, which we term octupole-driven spin-transfer torque (OTT). We demonstrate current-induced OTT switching of PtMn3|MgO|PtMn3 AFMTJs, fabricated on a thermally oxidized silicon substrate, exhibiting a record-high TMR value of 363% at room temperature and switching current densities of the order of 10 MA/cm2. Our theoretical modeling explains the origin of OTT in terms of the imbalance between intra- and inter-sublattice spin currents across the AFMTJ, and equivalently, in terms of the non-zero net cluster octupole polarization of each PtMn3 layer. This work establishes a new materials platform for antiferromagnetic spintronics and provides a pathway towards deeply scaled magnetic memory and room-temperature terahertz technologies.
title Octupole-driven spin-transfer torque switching of all-antiferromagnetic tunnel junctions
topic Materials Science
Mesoscale and Nanoscale Physics
Applied Physics
url https://arxiv.org/abs/2509.03026