Frustration-enhanced persistent currents in correlated trimer nanorings

Fuente: arXiv
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Main Authors: Fang, Tie-Feng, Lu, Wei-Tao, Guo, Ai-Min, Sun, Qing-Feng
Format: Preprint
Published: 2025
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author Fang, Tie-Feng
Lu, Wei-Tao
Guo, Ai-Min
Sun, Qing-Feng
author_facet Fang, Tie-Feng
Lu, Wei-Tao
Guo, Ai-Min
Sun, Qing-Feng
contents We investigate the persistent current in a correlated trimer nanoring comprising of three magnetic atoms, which sits on a metallic host and encloses a magnetic flux. In the molecular-orbital regime, charge fluctuations can reverse the aromaticity of the trimer molecule by driving quantum phase transitions between many-body states. It is shown that in frustrated trimers the superexchange-induced current as a function of interatom hopping is enhanced by the competition of conflicting magnetic orders, with an asymmetric peak at the quantum criticality separating the ferromagnetic and antiferromagnetic Kondo regimes. Interestingly, the critical current undergoes an anomalous rise with temperature before decaying, signaling the suppression of Kondo bound state at finite temperature. Our results demonstrate that the coherent current response to external flux indeed conveys important information on the states of strongly correlated systems.
format Preprint
id arxiv_https___arxiv_org_abs_2509_03924
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Frustration-enhanced persistent currents in correlated trimer nanorings
Fang, Tie-Feng
Lu, Wei-Tao
Guo, Ai-Min
Sun, Qing-Feng
Strongly Correlated Electrons
We investigate the persistent current in a correlated trimer nanoring comprising of three magnetic atoms, which sits on a metallic host and encloses a magnetic flux. In the molecular-orbital regime, charge fluctuations can reverse the aromaticity of the trimer molecule by driving quantum phase transitions between many-body states. It is shown that in frustrated trimers the superexchange-induced current as a function of interatom hopping is enhanced by the competition of conflicting magnetic orders, with an asymmetric peak at the quantum criticality separating the ferromagnetic and antiferromagnetic Kondo regimes. Interestingly, the critical current undergoes an anomalous rise with temperature before decaying, signaling the suppression of Kondo bound state at finite temperature. Our results demonstrate that the coherent current response to external flux indeed conveys important information on the states of strongly correlated systems.
title Frustration-enhanced persistent currents in correlated trimer nanorings
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2509.03924