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Main Authors: Hirler, Michael, Antonov, Alexander A., Baù, Enrico, Aigner, Andreas, Heimig, Connor, Hu, Haiyang, Tittl, Andreas
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2509.04896
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author Hirler, Michael
Antonov, Alexander A.
Baù, Enrico
Aigner, Andreas
Heimig, Connor
Hu, Haiyang
Tittl, Andreas
author_facet Hirler, Michael
Antonov, Alexander A.
Baù, Enrico
Aigner, Andreas
Heimig, Connor
Hu, Haiyang
Tittl, Andreas
contents Optical metasurfaces supporting resonances with high quality factors offer an outstanding platform for applications such as non-linear optics, light guiding, lasing, sensing, light-matter coupling, and quantum optics. However, their experimental realization typically demands elaborate multi-step procedures such as metal or dielectric deposition, lift-off, and reactive ion etching. As a consequence, accessibility, large-scale production and sustainability are constrained by reliance on cost-, time- and labor-intensive facilities. We overcome this fabrication hurdle by repurposing polymethyl methacrylate-which is usually employed as a temporary resist-as the resonator material, thereby eliminating all steps except for spin-coating, exposure and development. Because the low refractive index of the polymer limits effective mode formation, we present a bilayer recipe that enables the convenient fabrication of a freestanding membrane to maximize the index contrast with its surroundings. Since etching induced defects are circumvented, the membrane features high quality nanopatterns. We further examine the suspended membrane with scanning electron microscopy and extract its position-dependent spring constant and pretension with nanoindentation experiments applied by the tip of an atomic force microscope. Our all-polymer metasurface hosting Bound States in the Continuum experimentally delivers high quality factors (up to 523) at visible and near infrared wavelengths, despite the low refractive index of the polymer, and enables straightforward geometry-based tuning of both linewidth and resonance position. We envision this methodology to lay the groundwork for accessible, high performance metasurfaces with unique use cases such as material blending, angled writing and mechanically based resonance tuning.
format Preprint
id arxiv_https___arxiv_org_abs_2509_04896
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Accessible, All-Polymer Metasurfaces: Low Effort, High Quality Factor
Hirler, Michael
Antonov, Alexander A.
Baù, Enrico
Aigner, Andreas
Heimig, Connor
Hu, Haiyang
Tittl, Andreas
Optics
Optical metasurfaces supporting resonances with high quality factors offer an outstanding platform for applications such as non-linear optics, light guiding, lasing, sensing, light-matter coupling, and quantum optics. However, their experimental realization typically demands elaborate multi-step procedures such as metal or dielectric deposition, lift-off, and reactive ion etching. As a consequence, accessibility, large-scale production and sustainability are constrained by reliance on cost-, time- and labor-intensive facilities. We overcome this fabrication hurdle by repurposing polymethyl methacrylate-which is usually employed as a temporary resist-as the resonator material, thereby eliminating all steps except for spin-coating, exposure and development. Because the low refractive index of the polymer limits effective mode formation, we present a bilayer recipe that enables the convenient fabrication of a freestanding membrane to maximize the index contrast with its surroundings. Since etching induced defects are circumvented, the membrane features high quality nanopatterns. We further examine the suspended membrane with scanning electron microscopy and extract its position-dependent spring constant and pretension with nanoindentation experiments applied by the tip of an atomic force microscope. Our all-polymer metasurface hosting Bound States in the Continuum experimentally delivers high quality factors (up to 523) at visible and near infrared wavelengths, despite the low refractive index of the polymer, and enables straightforward geometry-based tuning of both linewidth and resonance position. We envision this methodology to lay the groundwork for accessible, high performance metasurfaces with unique use cases such as material blending, angled writing and mechanically based resonance tuning.
title Accessible, All-Polymer Metasurfaces: Low Effort, High Quality Factor
topic Optics
url https://arxiv.org/abs/2509.04896