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Main Authors: Zhong, Jianqi, Geng, Songyuan, Ying, Teng-Fei, Li, Haoxiang, Zhou, Benjamin T.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2509.05958
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author Zhong, Jianqi
Geng, Songyuan
Ying, Teng-Fei
Li, Haoxiang
Zhou, Benjamin T.
author_facet Zhong, Jianqi
Geng, Songyuan
Ying, Teng-Fei
Li, Haoxiang
Zhou, Benjamin T.
contents The long-sought dice lattice flat band has recently been discovered for the first time in two-dimensional layered electride yttrium monochloride (YCl) [Nature Communications 17, 2213 (2026)]. While essential flat band features of YCl were captured by an idealized simple dice lattice model, we reveal in this Letter that a unique layer-orbital-valley coupling in YCl puts up a fundamental obstruction against a simple three-band dice lattice description of the flat band, and necessitates a multi-orbital description that faithfully represents the symmetry, topology, and correlation physics in the first-ever dice metal. Using an ab initio based multi-orbital Hubbard model with local interactions, we predict that the multi-orbital flat band supports a robust ferromagnetic ground state and electrically tunable correlated quantum anomalous Hall phases that are absent in an interacting single-orbital dice lattice. Our findings open a new avenue for exploring correlation and topology in electride systems.
format Preprint
id arxiv_https___arxiv_org_abs_2509_05958
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle YCl Electride as a Multi-Orbital Correlated Topological Dice Lattice System
Zhong, Jianqi
Geng, Songyuan
Ying, Teng-Fei
Li, Haoxiang
Zhou, Benjamin T.
Materials Science
Strongly Correlated Electrons
The long-sought dice lattice flat band has recently been discovered for the first time in two-dimensional layered electride yttrium monochloride (YCl) [Nature Communications 17, 2213 (2026)]. While essential flat band features of YCl were captured by an idealized simple dice lattice model, we reveal in this Letter that a unique layer-orbital-valley coupling in YCl puts up a fundamental obstruction against a simple three-band dice lattice description of the flat band, and necessitates a multi-orbital description that faithfully represents the symmetry, topology, and correlation physics in the first-ever dice metal. Using an ab initio based multi-orbital Hubbard model with local interactions, we predict that the multi-orbital flat band supports a robust ferromagnetic ground state and electrically tunable correlated quantum anomalous Hall phases that are absent in an interacting single-orbital dice lattice. Our findings open a new avenue for exploring correlation and topology in electride systems.
title YCl Electride as a Multi-Orbital Correlated Topological Dice Lattice System
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2509.05958