Study of the elusive $5s-4f$ level crossing in highly charged osmium with optical transitions suitable for physics beyond the Standard Model searches

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Main Authors: Rehbehn, Nils-Holger, Sajith, Lakshmi Priya Kozhiparambil, Rosner, Michael K., Cheung, Charles, Porsev, Sergey G., Safronova, Marianna S., Worm, Steven, Budker, Dmitry, Pfeifer, Thomas, López-Urrutia, José R. Crespo, Bekker, Hendrik
Format: Preprint
Published: 2025
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author Rehbehn, Nils-Holger
Sajith, Lakshmi Priya Kozhiparambil
Rosner, Michael K.
Cheung, Charles
Porsev, Sergey G.
Safronova, Marianna S.
Worm, Steven
Budker, Dmitry
Pfeifer, Thomas
López-Urrutia, José R. Crespo
Bekker, Hendrik
author_facet Rehbehn, Nils-Holger
Sajith, Lakshmi Priya Kozhiparambil
Rosner, Michael K.
Cheung, Charles
Porsev, Sergey G.
Safronova, Marianna S.
Worm, Steven
Budker, Dmitry
Pfeifer, Thomas
López-Urrutia, José R. Crespo
Bekker, Hendrik
contents Optical transitions of highly charged ions can be very sensitive to hypothetical beyond-the-Standard-Model phenomena. Those near the $5s-4f$ level crossing, where the $5s$ and $4f$ are degenerate are especially promising. We present predictions from atomic theory and measurements of Os$^{15,16,17+}$ at an electron beam ion trap for identification of several transitions suitable for searches for a hypothetical fifth force and possible violations of local Lorentz invariance. The electric quadrupole (E2) transitions of Os$^{16+}$ that were found are especially suitable for frequency metrology due to their small linewidth of 44 $μ$Hz. Our calculations show the need for including enough inner-shell excitations to predict transition rates between configurations, which can otherwise be overestimated. Ultimately, the predicted interconfiguration transitions were too weak to be detected.
format Preprint
id arxiv_https___arxiv_org_abs_2509_06710
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Study of the elusive $5s-4f$ level crossing in highly charged osmium with optical transitions suitable for physics beyond the Standard Model searches
Rehbehn, Nils-Holger
Sajith, Lakshmi Priya Kozhiparambil
Rosner, Michael K.
Cheung, Charles
Porsev, Sergey G.
Safronova, Marianna S.
Worm, Steven
Budker, Dmitry
Pfeifer, Thomas
López-Urrutia, José R. Crespo
Bekker, Hendrik
Atomic Physics
Optical transitions of highly charged ions can be very sensitive to hypothetical beyond-the-Standard-Model phenomena. Those near the $5s-4f$ level crossing, where the $5s$ and $4f$ are degenerate are especially promising. We present predictions from atomic theory and measurements of Os$^{15,16,17+}$ at an electron beam ion trap for identification of several transitions suitable for searches for a hypothetical fifth force and possible violations of local Lorentz invariance. The electric quadrupole (E2) transitions of Os$^{16+}$ that were found are especially suitable for frequency metrology due to their small linewidth of 44 $μ$Hz. Our calculations show the need for including enough inner-shell excitations to predict transition rates between configurations, which can otherwise be overestimated. Ultimately, the predicted interconfiguration transitions were too weak to be detected.
title Study of the elusive $5s-4f$ level crossing in highly charged osmium with optical transitions suitable for physics beyond the Standard Model searches
topic Atomic Physics
url https://arxiv.org/abs/2509.06710