DEQuify your force field: More efficient simulations using deep equilibrium models

Fuente: arXiv
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Main Authors: Burger, Andreas, Thiede, Luca, Aspuru-Guzik, Alán, Vijaykumar, Nandita
Format: Preprint
Published: 2025
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author Burger, Andreas
Thiede, Luca
Aspuru-Guzik, Alán
Vijaykumar, Nandita
author_facet Burger, Andreas
Thiede, Luca
Aspuru-Guzik, Alán
Vijaykumar, Nandita
contents Machine learning force fields show great promise in enabling more accurate molecular dynamics simulations compared to manually derived ones. Much of the progress in recent years was driven by exploiting prior knowledge about physical systems, in particular symmetries under rotation, translation, and reflections. In this paper, we argue that there is another important piece of prior information that, thus fa,r hasn't been explored: Simulating a molecular system is necessarily continuous, and successive states are therefore extremely similar. Our contribution is to show that we can exploit this information by recasting a state-of-the-art equivariant base model as a deep equilibrium model. This allows us to recycle intermediate neural network features from previous time steps, enabling us to improve both accuracy and speed by $10\%-20\%$ on the MD17, MD22, and OC20 200k datasets, compared to the non-DEQ base model. The training is also much more memory efficient, allowing us to train more expressive models on larger systems.
format Preprint
id arxiv_https___arxiv_org_abs_2509_08734
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle DEQuify your force field: More efficient simulations using deep equilibrium models
Burger, Andreas
Thiede, Luca
Aspuru-Guzik, Alán
Vijaykumar, Nandita
Machine Learning
Artificial Intelligence
Machine learning force fields show great promise in enabling more accurate molecular dynamics simulations compared to manually derived ones. Much of the progress in recent years was driven by exploiting prior knowledge about physical systems, in particular symmetries under rotation, translation, and reflections. In this paper, we argue that there is another important piece of prior information that, thus fa,r hasn't been explored: Simulating a molecular system is necessarily continuous, and successive states are therefore extremely similar. Our contribution is to show that we can exploit this information by recasting a state-of-the-art equivariant base model as a deep equilibrium model. This allows us to recycle intermediate neural network features from previous time steps, enabling us to improve both accuracy and speed by $10\%-20\%$ on the MD17, MD22, and OC20 200k datasets, compared to the non-DEQ base model. The training is also much more memory efficient, allowing us to train more expressive models on larger systems.
title DEQuify your force field: More efficient simulations using deep equilibrium models
topic Machine Learning
Artificial Intelligence
url https://arxiv.org/abs/2509.08734