Realization of a Spin-1/2 Hexagonal-Plaquette Chain with Ising-Like Anisotropy

Fuente: arXiv
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Main Authors: Yamaguchi, Hironori, Furuya, Shunsuke C., Tominaga, Yu, Araki, Koji, Hagiwara, Masayuki
Format: Preprint
Published: 2025
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author Yamaguchi, Hironori
Furuya, Shunsuke C.
Tominaga, Yu
Araki, Koji
Hagiwara, Masayuki
author_facet Yamaguchi, Hironori
Furuya, Shunsuke C.
Tominaga, Yu
Araki, Koji
Hagiwara, Masayuki
contents We present the realization of a spin-1/2 hexagonal-plaquette chain with Ising anisotropy, an unexplored quantum spin model that serves as a platform for investigating anisotropic quantum magnetism. Specific heat at zero field reveals a sharp peak at $T_{\rm{N}}$ = 1.0 K, indicating a phase transition to a N$\acute{\rm{e}}$el order stabilized by interchain couplings. A perturbative analysis maps the system onto an effective spin-1/2 Ising-like chain, supporting the presence of an anisotropy-induced excitation gap. Furthermore, the interchain interactions may induce discrete excitations in the spinon continuum, reminiscent of Zeeman ladder physics observed in related 1D Ising-like systems. These results establish a well-defined model system for correlated spin phenomena in anisotropic magnets and highlight a route for engineering Ising-like quantum states in molecular-based frameworks.
format Preprint
id arxiv_https___arxiv_org_abs_2509_09060
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Realization of a Spin-1/2 Hexagonal-Plaquette Chain with Ising-Like Anisotropy
Yamaguchi, Hironori
Furuya, Shunsuke C.
Tominaga, Yu
Araki, Koji
Hagiwara, Masayuki
Strongly Correlated Electrons
We present the realization of a spin-1/2 hexagonal-plaquette chain with Ising anisotropy, an unexplored quantum spin model that serves as a platform for investigating anisotropic quantum magnetism. Specific heat at zero field reveals a sharp peak at $T_{\rm{N}}$ = 1.0 K, indicating a phase transition to a N$\acute{\rm{e}}$el order stabilized by interchain couplings. A perturbative analysis maps the system onto an effective spin-1/2 Ising-like chain, supporting the presence of an anisotropy-induced excitation gap. Furthermore, the interchain interactions may induce discrete excitations in the spinon continuum, reminiscent of Zeeman ladder physics observed in related 1D Ising-like systems. These results establish a well-defined model system for correlated spin phenomena in anisotropic magnets and highlight a route for engineering Ising-like quantum states in molecular-based frameworks.
title Realization of a Spin-1/2 Hexagonal-Plaquette Chain with Ising-Like Anisotropy
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2509.09060