Multi-Dimensional Photon-Correlations Reveal Triexciton Features in Single Perovskite Quantum Dots

Fuente: arXiv
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Main Authors: Hinkle, Alex, Tsao, Chieh, Duell, Adam, Utzat, Hendrik
Format: Preprint
Published: 2025
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author Hinkle, Alex
Tsao, Chieh
Duell, Adam
Utzat, Hendrik
author_facet Hinkle, Alex
Tsao, Chieh
Duell, Adam
Utzat, Hendrik
contents Lead-halide perovskite quantum dots (PQDs) are established quantum emitters with potential for entangled photon-pair generation via multiexciton cascades. However, the energetics and dynamics of many-body excitations remain poorly understood. Here, we perform time- and frequency-resolved photon-correlation spectroscopy of single CsPbBr\textsubscript{3} PQDs at low temperatures using a single-photon avalanche diode (SPAD) array detector. We report biexciton binding energies and assign their charged states, which undergo fast ($μ$s) switching dynamics. Most notably, we identify a spectral feature blue-shifted from the exciton by $7.4 \pm 1.9$ meV as the bound triexciton and establish the order of its cascade emission. These results highlight the power of low-temperature, multidimensional photon-correlation spectroscopy for resolving complex many-body dynamics.
format Preprint
id arxiv_https___arxiv_org_abs_2509_12461
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Multi-Dimensional Photon-Correlations Reveal Triexciton Features in Single Perovskite Quantum Dots
Hinkle, Alex
Tsao, Chieh
Duell, Adam
Utzat, Hendrik
Materials Science
Lead-halide perovskite quantum dots (PQDs) are established quantum emitters with potential for entangled photon-pair generation via multiexciton cascades. However, the energetics and dynamics of many-body excitations remain poorly understood. Here, we perform time- and frequency-resolved photon-correlation spectroscopy of single CsPbBr\textsubscript{3} PQDs at low temperatures using a single-photon avalanche diode (SPAD) array detector. We report biexciton binding energies and assign their charged states, which undergo fast ($μ$s) switching dynamics. Most notably, we identify a spectral feature blue-shifted from the exciton by $7.4 \pm 1.9$ meV as the bound triexciton and establish the order of its cascade emission. These results highlight the power of low-temperature, multidimensional photon-correlation spectroscopy for resolving complex many-body dynamics.
title Multi-Dimensional Photon-Correlations Reveal Triexciton Features in Single Perovskite Quantum Dots
topic Materials Science
url https://arxiv.org/abs/2509.12461