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Autori principali: Noskov, Aleksei I., Kotlyar, Alexander B., Potma, Eric O., Fishman, Dmitry A.
Natura: Preprint
Pubblicazione: 2025
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Accesso online:https://arxiv.org/abs/2509.12690
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author Noskov, Aleksei I.
Kotlyar, Alexander B.
Potma, Eric O.
Fishman, Dmitry A.
author_facet Noskov, Aleksei I.
Kotlyar, Alexander B.
Potma, Eric O.
Fishman, Dmitry A.
contents Silicon indirect bandgap fundamentally limits its ability to emit light, hindering the development of silicon-based light sources. Here, we explore a conceptually new solution to this long-standing challenge. We demonstrate ultrabroadband photo- and electroluminescence from bulk silicon, enabled by a radiative pathway mediated by momentum-expanded photonic states that bypass phonon-assisted transitions. This mechanism, previously demonstrated using metallic nanoparticles as photon confiners, is here realized in an all-silicon system using embedded sub-1.5 nm silicon nanoparticles. Since such ultrasmall particles possess negligible intrinsic emission efficiency, we instead demonstrate that they act as photonic confiners, enabling radiative recombination in the surrounding bulk material. The agreement with prior metal-based systems confirms that confinement size, rather than material composition, governs the activation of radiative transitions in a momentum-forbidden system. The emission spans the visible to near-infrared spectral range, with electroluminescence in an undoped semiconductor device visible under ambient conditions and a quantum efficiency estimated as ~0.2%. These findings establish a new route to efficient light emission in silicon and reveal a hybrid light-matter regime in which extreme photonic confinement reshapes the electronic transition landscape.
format Preprint
id arxiv_https___arxiv_org_abs_2509_12690
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Broadband Photo- and Electroluminescence from Bulk Silicon via Strong Photonic Confinement
Noskov, Aleksei I.
Kotlyar, Alexander B.
Potma, Eric O.
Fishman, Dmitry A.
Optics
Silicon indirect bandgap fundamentally limits its ability to emit light, hindering the development of silicon-based light sources. Here, we explore a conceptually new solution to this long-standing challenge. We demonstrate ultrabroadband photo- and electroluminescence from bulk silicon, enabled by a radiative pathway mediated by momentum-expanded photonic states that bypass phonon-assisted transitions. This mechanism, previously demonstrated using metallic nanoparticles as photon confiners, is here realized in an all-silicon system using embedded sub-1.5 nm silicon nanoparticles. Since such ultrasmall particles possess negligible intrinsic emission efficiency, we instead demonstrate that they act as photonic confiners, enabling radiative recombination in the surrounding bulk material. The agreement with prior metal-based systems confirms that confinement size, rather than material composition, governs the activation of radiative transitions in a momentum-forbidden system. The emission spans the visible to near-infrared spectral range, with electroluminescence in an undoped semiconductor device visible under ambient conditions and a quantum efficiency estimated as ~0.2%. These findings establish a new route to efficient light emission in silicon and reveal a hybrid light-matter regime in which extreme photonic confinement reshapes the electronic transition landscape.
title Broadband Photo- and Electroluminescence from Bulk Silicon via Strong Photonic Confinement
topic Optics
url https://arxiv.org/abs/2509.12690