Ultrafast optically induced tunneling in narrow metallic gaps from the time dependent density functional perspective

Fuente: arXiv
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Autori principali: Ma, Boyang, Babaze, Antton, Krüger, Michael, Aizpurua, Javier, Borisov, Andrei G.
Natura: Preprint
Pubblicazione: 2025
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author Ma, Boyang
Babaze, Antton
Krüger, Michael
Aizpurua, Javier
Borisov, Andrei G.
author_facet Ma, Boyang
Babaze, Antton
Krüger, Michael
Aizpurua, Javier
Borisov, Andrei G.
contents In this work, using the time-dependent density functional theory, we address the electron tunneling triggered by short (single-cycle and several-cycle) optical pulses in narrow metallic gaps under conditions relevant for actual experiments. We identify photon-assisted tunneling with one-photon, two-photon, and higher-order photon absorption, and we discuss the effect of the tunneling barrier, applied bias, and strength of the optical field on transition from photon-assisted tunneling (weak optical fields) to the optical field emission at strong optical fields. The numerical single-electron calculations and an analytical strong-field theory model are used to gain deeper insights into the results of the time-dependent density functional theory calculations. Additionally, our parameter-free calculations allow us to retrieve and explain recent experimental results on optically induced transport in narrow metallic gaps under an applied dc bias.
format Preprint
id arxiv_https___arxiv_org_abs_2509_14802
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Ultrafast optically induced tunneling in narrow metallic gaps from the time dependent density functional perspective
Ma, Boyang
Babaze, Antton
Krüger, Michael
Aizpurua, Javier
Borisov, Andrei G.
Optics
In this work, using the time-dependent density functional theory, we address the electron tunneling triggered by short (single-cycle and several-cycle) optical pulses in narrow metallic gaps under conditions relevant for actual experiments. We identify photon-assisted tunneling with one-photon, two-photon, and higher-order photon absorption, and we discuss the effect of the tunneling barrier, applied bias, and strength of the optical field on transition from photon-assisted tunneling (weak optical fields) to the optical field emission at strong optical fields. The numerical single-electron calculations and an analytical strong-field theory model are used to gain deeper insights into the results of the time-dependent density functional theory calculations. Additionally, our parameter-free calculations allow us to retrieve and explain recent experimental results on optically induced transport in narrow metallic gaps under an applied dc bias.
title Ultrafast optically induced tunneling in narrow metallic gaps from the time dependent density functional perspective
topic Optics
url https://arxiv.org/abs/2509.14802