Sub-tesla on-chip nanomagnetic metamaterial platform for angle-resolved photoemission spectroscopy

Fuente: arXiv
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Main Authors: Li, Wenxin, Wanichwecharungruang, Wisha, Guo, Mingyang, Chioar, Ioan-Augustin, Nandakumaran, Nileena, Ramberger, Justin, Li, Senlei, Kang, Zhibo, Yang, Jinming, Lu, Donghui, Hashimoto, Makoto, Du, Chunhui Rita, Leighton, Chris, Schiffer, Peter, Ma, Qiong, Yi, Ming, He, Yu
Format: Preprint
Published: 2025
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author Li, Wenxin
Wanichwecharungruang, Wisha
Guo, Mingyang
Chioar, Ioan-Augustin
Nandakumaran, Nileena
Ramberger, Justin
Li, Senlei
Kang, Zhibo
Yang, Jinming
Lu, Donghui
Hashimoto, Makoto
Du, Chunhui Rita
Leighton, Chris
Schiffer, Peter
Ma, Qiong
Yi, Ming
He, Yu
author_facet Li, Wenxin
Wanichwecharungruang, Wisha
Guo, Mingyang
Chioar, Ioan-Augustin
Nandakumaran, Nileena
Ramberger, Justin
Li, Senlei
Kang, Zhibo
Yang, Jinming
Lu, Donghui
Hashimoto, Makoto
Du, Chunhui Rita
Leighton, Chris
Schiffer, Peter
Ma, Qiong
Yi, Ming
He, Yu
contents Magnetically controlled states in quantum materials are central to their unique electronic and magnetic properties. However, direct momentum-resolved visualization of these states via angle-resolved photoemission spectroscopy (ARPES) has been hindered by the disruptive effect of magnetic fields on photoelectron trajectories. Here, we introduce an \textit{in-situ} method that is, in principle, capable of applying magnetic fields up to 1 T. This method uses substrates composed of nanomagnetic metamaterial arrays with alternating polarity. Such substrates can generate strong, homogeneous, and spatially confined fields applicable to samples with thicknesses up to the micron scale, enabling ARPES measurements under magnetic fields with minimal photoelectron trajectory distortion. We demonstrate this minimal distortion with ARPES data taken on monolayer graphene. Our method paves the way for probing magnetic field-dependent electronic structures and studying field-tunable quantum phases with state-of-the-art energy-momentum resolutions.
format Preprint
id arxiv_https___arxiv_org_abs_2509_15092
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Sub-tesla on-chip nanomagnetic metamaterial platform for angle-resolved photoemission spectroscopy
Li, Wenxin
Wanichwecharungruang, Wisha
Guo, Mingyang
Chioar, Ioan-Augustin
Nandakumaran, Nileena
Ramberger, Justin
Li, Senlei
Kang, Zhibo
Yang, Jinming
Lu, Donghui
Hashimoto, Makoto
Du, Chunhui Rita
Leighton, Chris
Schiffer, Peter
Ma, Qiong
Yi, Ming
He, Yu
Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
Magnetically controlled states in quantum materials are central to their unique electronic and magnetic properties. However, direct momentum-resolved visualization of these states via angle-resolved photoemission spectroscopy (ARPES) has been hindered by the disruptive effect of magnetic fields on photoelectron trajectories. Here, we introduce an \textit{in-situ} method that is, in principle, capable of applying magnetic fields up to 1 T. This method uses substrates composed of nanomagnetic metamaterial arrays with alternating polarity. Such substrates can generate strong, homogeneous, and spatially confined fields applicable to samples with thicknesses up to the micron scale, enabling ARPES measurements under magnetic fields with minimal photoelectron trajectory distortion. We demonstrate this minimal distortion with ARPES data taken on monolayer graphene. Our method paves the way for probing magnetic field-dependent electronic structures and studying field-tunable quantum phases with state-of-the-art energy-momentum resolutions.
title Sub-tesla on-chip nanomagnetic metamaterial platform for angle-resolved photoemission spectroscopy
topic Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2509.15092