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Bibliographic Details
Main Authors: Zhang, Yichen, Jeong, Seung Gyo, Buiarelli, Luca, Lee, Seungjun, Guo, Yucheng, Wen, Jiaqin, Li, Hang, Nair, Sreejith, Choi, In Hyeok, Ren, Zheng, Yue, Ziqin, Fedorov, Alexei, Mo, Sung-Kwan, Kono, Junichiro, Lee, Jong Seok, Low, Tony, Birol, Turan, Fernandes, Rafael M., Radovic, Milan, Jalan, Bharat, Yi, Ming
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2509.16361
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Table of Contents:
  • Recently, rutile RuO$_2$ has attracted renewed interest due to expectations of prominent altermagnetic spin-splitting. However, accumulating experimental evidence suggests that in its bulk and thick-film forms, RuO$_2$ does not display any form of magnetic ordering. Despite this, the spin structure of RuO$_2$ remains largely unexplored in the ultra-thin limit, where substrate-imposed epitaxial strain can be substantial. Here, we employ spin-resolved angle-resolved photoemission spectroscopy, supported by ab-initio calculations, to reveal the electronic structure of 2.7~nm-thick epitaxial RuO$_2$ heterostructures. We observe an unconventional spin texture characterized by the coexistence of mirror-even and mirror-odd momentum-dependent components. A comprehensive symmetry analysis rules out nonmagnetic origins of this spin texture. These findings suggest an emergent non-relativistic spin structure enabled by epitaxial strain in the ultra-thin limit, marking a distinct departure from the behavior of relaxed or bulk RuO$_2$. Our work opens new perspectives for exploring symmetry-breaking mechanisms and spin textures in oxide heterostructures.