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Main Authors: Kihara, Takumi, Xu, Xiao, Ogi, Yuki, Adachi, Yoshiya, Roy, Tufan, Matsuura, Ryuji, Kanomata, Takeshi
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2509.17378
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author Kihara, Takumi
Xu, Xiao
Ogi, Yuki
Adachi, Yoshiya
Roy, Tufan
Matsuura, Ryuji
Kanomata, Takeshi
author_facet Kihara, Takumi
Xu, Xiao
Ogi, Yuki
Adachi, Yoshiya
Roy, Tufan
Matsuura, Ryuji
Kanomata, Takeshi
contents We investigated the magnetic and thermoelectric properties of the full Heusler alloy Co$_2$NbSn, which exhibits a martensitic transformation at 240 K. Magnetization measurements reveal weak itinerant ferromagnetism in the martensitic phase, which is well described by Takahashi's spin fluctuation theory. The characteristic spin fluctuation parameters were estimated to be T_0 = 1.0$\times$10^3 K and T_A = 7.2$\times$10^3 K. Seebeck coefficient measurements under magnetic fields up to 9 T show complex temperature and field dependence, which we decomposed into electron diffusion, spin fluctuation drag, and magnon drag components. A significant magnon-drag contribution was identified in both austenite and martensitic phases. Remarkably, this contribution is strongly enhanced in the martensitic phase compared to the austenite phase, despite a smaller magnetic moment. These findings provide evidence for robust low-energy spin excitations and highlight the potential of martensitic transformation in enhancing the thermoelectric performance of itinerant ferromagnetic alloys.
format Preprint
id arxiv_https___arxiv_org_abs_2509_17378
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Magnetically Enhanced Thermoelectric Effect Driven by Martensitic Transformation in the Weak Itinerant Ferromagnet Co$_2$NbSn
Kihara, Takumi
Xu, Xiao
Ogi, Yuki
Adachi, Yoshiya
Roy, Tufan
Matsuura, Ryuji
Kanomata, Takeshi
Materials Science
Strongly Correlated Electrons
We investigated the magnetic and thermoelectric properties of the full Heusler alloy Co$_2$NbSn, which exhibits a martensitic transformation at 240 K. Magnetization measurements reveal weak itinerant ferromagnetism in the martensitic phase, which is well described by Takahashi's spin fluctuation theory. The characteristic spin fluctuation parameters were estimated to be T_0 = 1.0$\times$10^3 K and T_A = 7.2$\times$10^3 K. Seebeck coefficient measurements under magnetic fields up to 9 T show complex temperature and field dependence, which we decomposed into electron diffusion, spin fluctuation drag, and magnon drag components. A significant magnon-drag contribution was identified in both austenite and martensitic phases. Remarkably, this contribution is strongly enhanced in the martensitic phase compared to the austenite phase, despite a smaller magnetic moment. These findings provide evidence for robust low-energy spin excitations and highlight the potential of martensitic transformation in enhancing the thermoelectric performance of itinerant ferromagnetic alloys.
title Magnetically Enhanced Thermoelectric Effect Driven by Martensitic Transformation in the Weak Itinerant Ferromagnet Co$_2$NbSn
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2509.17378