Negative charge acquisition by isolated single microdroplets from plasma exposure at atmospheric pressure

Fuente: arXiv
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Auteurs principaux: Hendawy, Nourhan, McQuaid, Harold, Uidhir, Somhairle Mag, Rutherford, David, Diver, Declan, Mariotti, Davide, Maguire, Paul
Format: Preprint
Publié: 2025
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author Hendawy, Nourhan
McQuaid, Harold
Uidhir, Somhairle Mag
Rutherford, David
Diver, Declan
Mariotti, Davide
Maguire, Paul
author_facet Hendawy, Nourhan
McQuaid, Harold
Uidhir, Somhairle Mag
Rutherford, David
Diver, Declan
Mariotti, Davide
Maguire, Paul
contents Charged liquid microdroplets have generated significant interest recently due to the observation of chemical reaction rate enhancement by orders of magnitude. Droplet charging by plasma irradiation has been observed along with significantly enhanced reaction rates in liquid. In this paper we measure the charge on fixed size (47 $μ$m) individual droplets, exposed for approximately 4 ms to a low temperature RF-driven plasma operated at atmospheric pressure. The measured charge values (0.8 - 2.0 $\times 10^{7}$ electrons) approached the Rayleigh limit for the given droplet diameter. Results were compared with finite element simulations of plasma charging which provided estimates of surface electric fields and charge fluxes to the droplet surface and helps advance the development of a theoretical framework for plasma-charged microreactors.
format Preprint
id arxiv_https___arxiv_org_abs_2509_17379
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Negative charge acquisition by isolated single microdroplets from plasma exposure at atmospheric pressure
Hendawy, Nourhan
McQuaid, Harold
Uidhir, Somhairle Mag
Rutherford, David
Diver, Declan
Mariotti, Davide
Maguire, Paul
Plasma Physics
Charged liquid microdroplets have generated significant interest recently due to the observation of chemical reaction rate enhancement by orders of magnitude. Droplet charging by plasma irradiation has been observed along with significantly enhanced reaction rates in liquid. In this paper we measure the charge on fixed size (47 $μ$m) individual droplets, exposed for approximately 4 ms to a low temperature RF-driven plasma operated at atmospheric pressure. The measured charge values (0.8 - 2.0 $\times 10^{7}$ electrons) approached the Rayleigh limit for the given droplet diameter. Results were compared with finite element simulations of plasma charging which provided estimates of surface electric fields and charge fluxes to the droplet surface and helps advance the development of a theoretical framework for plasma-charged microreactors.
title Negative charge acquisition by isolated single microdroplets from plasma exposure at atmospheric pressure
topic Plasma Physics
url https://arxiv.org/abs/2509.17379