Data-driven optimization of pixelated CdZnTe spectrometers for uranium enrichment assay

Fuente: arXiv
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Autores principales: Vavrek, Jayson R., MacDonald, Thomas D., Parrilla, Hannah S., Deshmukh, Nikhil S., Zalavadia, Mital A., McDonald, Benjamin S.
Formato: Preprint
Publicado: 2025
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author Vavrek, Jayson R.
MacDonald, Thomas D.
Parrilla, Hannah S.
Deshmukh, Nikhil S.
Zalavadia, Mital A.
McDonald, Benjamin S.
author_facet Vavrek, Jayson R.
MacDonald, Thomas D.
Parrilla, Hannah S.
Deshmukh, Nikhil S.
Zalavadia, Mital A.
McDonald, Benjamin S.
contents In recent work [Vavrek et al. (2025)], we developed the performance optimization framework spectre-ml for gamma spectrometers with variable performance across many readout channels. The framework uses non-negative matrix factorization (NMF) and clustering to learn groups of similarly-performing channels and sweep through various learned channel combinations to optimize the performance tradeoff of including worse-performing channels for better total efficiency. In this work, we integrate the pyGEM uranium enrichment assay code with our spectre-ml framework, and show that the U-235 enrichment relative uncertainty can be directly used as an optimization target. We find that this optimization reduces relative uncertainties after a 30-minute measurement by an average of 20%, as tested on six different H3D M400 CdZnTe spectrometers, which can significantly improve uranium non-destructive assay measurement times in nuclear safeguards contexts. Additionally, this work demonstrates that the spectre-ml optimization framework can accommodate arbitrary end-user spectroscopic analysis code and performance metrics, enabling future optimizations for complex Pu spectra.
format Preprint
id arxiv_https___arxiv_org_abs_2509_18517
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Data-driven optimization of pixelated CdZnTe spectrometers for uranium enrichment assay
Vavrek, Jayson R.
MacDonald, Thomas D.
Parrilla, Hannah S.
Deshmukh, Nikhil S.
Zalavadia, Mital A.
McDonald, Benjamin S.
Instrumentation and Detectors
In recent work [Vavrek et al. (2025)], we developed the performance optimization framework spectre-ml for gamma spectrometers with variable performance across many readout channels. The framework uses non-negative matrix factorization (NMF) and clustering to learn groups of similarly-performing channels and sweep through various learned channel combinations to optimize the performance tradeoff of including worse-performing channels for better total efficiency. In this work, we integrate the pyGEM uranium enrichment assay code with our spectre-ml framework, and show that the U-235 enrichment relative uncertainty can be directly used as an optimization target. We find that this optimization reduces relative uncertainties after a 30-minute measurement by an average of 20%, as tested on six different H3D M400 CdZnTe spectrometers, which can significantly improve uranium non-destructive assay measurement times in nuclear safeguards contexts. Additionally, this work demonstrates that the spectre-ml optimization framework can accommodate arbitrary end-user spectroscopic analysis code and performance metrics, enabling future optimizations for complex Pu spectra.
title Data-driven optimization of pixelated CdZnTe spectrometers for uranium enrichment assay
topic Instrumentation and Detectors
url https://arxiv.org/abs/2509.18517