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Auteurs principaux: Huang, Jian, Aghabozorgi, Fatemeh, Brock, Stephanie
Format: Preprint
Publié: 2025
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Accès en ligne:https://arxiv.org/abs/2509.24131
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author Huang, Jian
Aghabozorgi, Fatemeh
Brock, Stephanie
author_facet Huang, Jian
Aghabozorgi, Fatemeh
Brock, Stephanie
contents We report magnetoelectric coupling in nanoparticle assemblies that persists to temperatures over 300 times lower than in previous studies. The ME response saturates at low temperature, revealing a quantum plateau of the coupling. A field dependence analysis shows a crossover from quadratic to linear behavior, captured by a phenomenological expansion $C(B,T) \simeq C_0(T) + a_1(T) B + a_2(T) B^2$. The magnitude of the extracted quadratic coefficient, $|a_2(T)|$, follows a power law $|a_2(T)| \sim T^{-α}$ with $α\approx 1.15$, indicating proximity to a quantum critical regime. The observed saturation reflects a new intrinsic energy scale, distinct from finite-size or extrinsic effects. These results establish nanoparticle assemblies as a new platform for studying quantum magnetoelectric phenomena.
format Preprint
id arxiv_https___arxiv_org_abs_2509_24131
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Quantum Saturation of Magnetoelectric Coupling in Fe$_3$O$_4$ Nanoparticles
Huang, Jian
Aghabozorgi, Fatemeh
Brock, Stephanie
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
We report magnetoelectric coupling in nanoparticle assemblies that persists to temperatures over 300 times lower than in previous studies. The ME response saturates at low temperature, revealing a quantum plateau of the coupling. A field dependence analysis shows a crossover from quadratic to linear behavior, captured by a phenomenological expansion $C(B,T) \simeq C_0(T) + a_1(T) B + a_2(T) B^2$. The magnitude of the extracted quadratic coefficient, $|a_2(T)|$, follows a power law $|a_2(T)| \sim T^{-α}$ with $α\approx 1.15$, indicating proximity to a quantum critical regime. The observed saturation reflects a new intrinsic energy scale, distinct from finite-size or extrinsic effects. These results establish nanoparticle assemblies as a new platform for studying quantum magnetoelectric phenomena.
title Quantum Saturation of Magnetoelectric Coupling in Fe$_3$O$_4$ Nanoparticles
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2509.24131