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Bibliographic Details
Main Authors: Huang, Jian, Aghabozorgi, Fatemeh, Brock, Stephanie
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2509.24131
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Table of Contents:
  • We report magnetoelectric coupling in nanoparticle assemblies that persists to temperatures over 300 times lower than in previous studies. The ME response saturates at low temperature, revealing a quantum plateau of the coupling. A field dependence analysis shows a crossover from quadratic to linear behavior, captured by a phenomenological expansion $C(B,T) \simeq C_0(T) + a_1(T) B + a_2(T) B^2$. The magnitude of the extracted quadratic coefficient, $|a_2(T)|$, follows a power law $|a_2(T)| \sim T^{-α}$ with $α\approx 1.15$, indicating proximity to a quantum critical regime. The observed saturation reflects a new intrinsic energy scale, distinct from finite-size or extrinsic effects. These results establish nanoparticle assemblies as a new platform for studying quantum magnetoelectric phenomena.