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Hauptverfasser: Weiss, Marvin Alexander, Schlegel, Julius, Anić, Daniel, Steiner, Emil, Herbst, Franz Stefan, Nakajima, Makoto, Kurihara, Takayuki, Leitenstorfer, Alfred, Nowak, Ulrich, Goennenwein, Sebastian T. B.
Format: Preprint
Veröffentlicht: 2025
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Online-Zugang:https://arxiv.org/abs/2509.26084
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author Weiss, Marvin Alexander
Schlegel, Julius
Anić, Daniel
Steiner, Emil
Herbst, Franz Stefan
Nakajima, Makoto
Kurihara, Takayuki
Leitenstorfer, Alfred
Nowak, Ulrich
Goennenwein, Sebastian T. B.
author_facet Weiss, Marvin Alexander
Schlegel, Julius
Anić, Daniel
Steiner, Emil
Herbst, Franz Stefan
Nakajima, Makoto
Kurihara, Takayuki
Leitenstorfer, Alfred
Nowak, Ulrich
Goennenwein, Sebastian T. B.
contents The properties of spin fluctuations in antiferromagnets are largely unexplored, in particular at ultrafast timescales. Here, we employ femtosecond noise correlation spectroscopy (FemNoC) to experimentally study magnetization fluctuations in the canted antiferromagnet Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$ across its spin reorientation transition and under external magnetic fields. By comparing our measurements to atomistic spin noise and Monte Carlo simulations, we find that the amplitude of the spin noise is governed by the free energy, with stronger fluctuations in regions where the potential landscape softens. We furthermore demonstrate that external magnetic fields suppress spin fluctuations and enhance the quasi-ferromagnetic magnon frequency by effectively stiffening the potential. These results highlight an effective route for tuning ultrafast magnetization fluctuations via external parameters.
format Preprint
id arxiv_https___arxiv_org_abs_2509_26084
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Field-tuning of ultrafast magnetization fluctuations in Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$
Weiss, Marvin Alexander
Schlegel, Julius
Anić, Daniel
Steiner, Emil
Herbst, Franz Stefan
Nakajima, Makoto
Kurihara, Takayuki
Leitenstorfer, Alfred
Nowak, Ulrich
Goennenwein, Sebastian T. B.
Materials Science
Optics
The properties of spin fluctuations in antiferromagnets are largely unexplored, in particular at ultrafast timescales. Here, we employ femtosecond noise correlation spectroscopy (FemNoC) to experimentally study magnetization fluctuations in the canted antiferromagnet Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$ across its spin reorientation transition and under external magnetic fields. By comparing our measurements to atomistic spin noise and Monte Carlo simulations, we find that the amplitude of the spin noise is governed by the free energy, with stronger fluctuations in regions where the potential landscape softens. We furthermore demonstrate that external magnetic fields suppress spin fluctuations and enhance the quasi-ferromagnetic magnon frequency by effectively stiffening the potential. These results highlight an effective route for tuning ultrafast magnetization fluctuations via external parameters.
title Field-tuning of ultrafast magnetization fluctuations in Sm$_{0.7}$Er$_{0.3}$FeO$_{3}$
topic Materials Science
Optics
url https://arxiv.org/abs/2509.26084