Four Moiré materials at One Magic Angle in Helical Quadrilayer Graphene

Fuente: arXiv
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Autores principales: Fujimoto, Manato, Nakatsuji, Naoto, Vishwanath, Ashvin, Ledwith, Patrick
Formato: Preprint
Publicado: 2025
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author Fujimoto, Manato
Nakatsuji, Naoto
Vishwanath, Ashvin
Ledwith, Patrick
author_facet Fujimoto, Manato
Nakatsuji, Naoto
Vishwanath, Ashvin
Ledwith, Patrick
contents We introduce helical twisted quadrilayer graphene (HTQG), four graphene sheets rotated by the same small angle, as a versatile and experimentally accessible platform for correlated topological matter. HTQG consists of three moiré lattices, formed by interference between adjacent graphene layers, that are twisted relative to each other. Lattice relaxation produces four types of large-scale commensurate domains. The domains are characterized by the stacking of the three moiré lattices and come in two types: Type-I "Bernal" stacking and Type-II "rhombohedral" stacking. Domain walls between adjacent stackings often host topologically protected edge states, forming networks at the supermoiré and super-supermoiré scales. Remarkably, all four moiré substructures have narrow bands at the same magic angle $θ\approx 2.3^\circ$, allowing their correlated phases to be simultaneously targeted in device manufacturing. We argue that the Type-I domains are especially suitable for realizing robust superconductivity which emerges from doping topological insulators, and Chern insulators in $C = \pm 2$ bands.
format Preprint
id arxiv_https___arxiv_org_abs_2510_02444
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Four Moiré materials at One Magic Angle in Helical Quadrilayer Graphene
Fujimoto, Manato
Nakatsuji, Naoto
Vishwanath, Ashvin
Ledwith, Patrick
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
We introduce helical twisted quadrilayer graphene (HTQG), four graphene sheets rotated by the same small angle, as a versatile and experimentally accessible platform for correlated topological matter. HTQG consists of three moiré lattices, formed by interference between adjacent graphene layers, that are twisted relative to each other. Lattice relaxation produces four types of large-scale commensurate domains. The domains are characterized by the stacking of the three moiré lattices and come in two types: Type-I "Bernal" stacking and Type-II "rhombohedral" stacking. Domain walls between adjacent stackings often host topologically protected edge states, forming networks at the supermoiré and super-supermoiré scales. Remarkably, all four moiré substructures have narrow bands at the same magic angle $θ\approx 2.3^\circ$, allowing their correlated phases to be simultaneously targeted in device manufacturing. We argue that the Type-I domains are especially suitable for realizing robust superconductivity which emerges from doping topological insulators, and Chern insulators in $C = \pm 2$ bands.
title Four Moiré materials at One Magic Angle in Helical Quadrilayer Graphene
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2510.02444