Thermal assisted transport of biexcitons in monolayer WSe2

Fuente: arXiv
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Autori principali: Béret, Dorian, Hemmen, Louka, Jindal, Vishwas, Raha, Sreyan, Amand, Thierry, Lagarde, Delphine, Balocchi, Andrea, Robert, Cédric, Carrere, Helene, Marie, Xavier, Renucci, Pierre, Lombez, Laurent
Natura: Preprint
Pubblicazione: 2025
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author Béret, Dorian
Hemmen, Louka
Jindal, Vishwas
Raha, Sreyan
Amand, Thierry
Lagarde, Delphine
Balocchi, Andrea
Robert, Cédric
Carrere, Helene
Marie, Xavier
Renucci, Pierre
Lombez, Laurent
author_facet Béret, Dorian
Hemmen, Louka
Jindal, Vishwas
Raha, Sreyan
Amand, Thierry
Lagarde, Delphine
Balocchi, Andrea
Robert, Cédric
Carrere, Helene
Marie, Xavier
Renucci, Pierre
Lombez, Laurent
contents Studies of excitonic transport in transition metal dichalcogenide monolayers have attracted increasing interest in recent years in order to develop nano-optoelectronic devices made with 2D materials. These studies began with low to moderate optical excitation regimes, and more recently have focused on high injection regimes where nonlinear effects appear. This article is focused on the transport of biexcitons by spatially and temporally resolved photoluminescence spectroscopy at high excitation flux. The study is carried out on a high-quality WSe$_2$ monolayer encapsulated in hexagonal boron nitride. The results show that a Seebeck current affects transport in connection with the presence of hot biexcitons. In particular, we observe the formation of spatial rings, also called halos, which have been observed in other excitonic gases. These results tend to generalize the importance of high-energy populations in excitonic transport in TMD, even for complex and heavy excitonic particles.
format Preprint
id arxiv_https___arxiv_org_abs_2510_03092
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Thermal assisted transport of biexcitons in monolayer WSe2
Béret, Dorian
Hemmen, Louka
Jindal, Vishwas
Raha, Sreyan
Amand, Thierry
Lagarde, Delphine
Balocchi, Andrea
Robert, Cédric
Carrere, Helene
Marie, Xavier
Renucci, Pierre
Lombez, Laurent
Materials Science
Studies of excitonic transport in transition metal dichalcogenide monolayers have attracted increasing interest in recent years in order to develop nano-optoelectronic devices made with 2D materials. These studies began with low to moderate optical excitation regimes, and more recently have focused on high injection regimes where nonlinear effects appear. This article is focused on the transport of biexcitons by spatially and temporally resolved photoluminescence spectroscopy at high excitation flux. The study is carried out on a high-quality WSe$_2$ monolayer encapsulated in hexagonal boron nitride. The results show that a Seebeck current affects transport in connection with the presence of hot biexcitons. In particular, we observe the formation of spatial rings, also called halos, which have been observed in other excitonic gases. These results tend to generalize the importance of high-energy populations in excitonic transport in TMD, even for complex and heavy excitonic particles.
title Thermal assisted transport of biexcitons in monolayer WSe2
topic Materials Science
url https://arxiv.org/abs/2510.03092