Probing frustrated metallo-molecular spin Kondo lattice interfaces through anomalous Nernst effect

Fuente: arXiv
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Autores principales: Ozdemir, Servet, Rogers, Matthew, McCluskey, Conor J., McQuaid, Raymond G., Parkin, Zachariah, Ali, Mannan, Burnell, Gavin, Barker, Joseph, Hickey, B J, Cespedes, Oscar
Formato: Preprint
Publicado: 2025
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author Ozdemir, Servet
Rogers, Matthew
McCluskey, Conor J.
McQuaid, Raymond G.
Parkin, Zachariah
Ali, Mannan
Burnell, Gavin
Barker, Joseph
Hickey, B J
Cespedes, Oscar
author_facet Ozdemir, Servet
Rogers, Matthew
McCluskey, Conor J.
McQuaid, Raymond G.
Parkin, Zachariah
Ali, Mannan
Burnell, Gavin
Barker, Joseph
Hickey, B J
Cespedes, Oscar
contents Frustrated Kondo spin lattice (KSL) systems away from the antiferromagnetic (AFM) ground state have been found to display strange metal behaviour. A signature of strange metals in correlated systems is large Nernst response. Metallo-molecular interfaces of supramolecular lattices have been demonstrated as 2D KSL systems in STM studies. Here going beyond STM experiments we report a frustrated AFM state on molecular interfaces of Pt(111) and Pt(111)/Co films with around room temperature spin freezing transitions. Near these transitions we measure an anomalous Nernst coefficient of at least 3 $μ$V/K.
format Preprint
id arxiv_https___arxiv_org_abs_2510_04824
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Probing frustrated metallo-molecular spin Kondo lattice interfaces through anomalous Nernst effect
Ozdemir, Servet
Rogers, Matthew
McCluskey, Conor J.
McQuaid, Raymond G.
Parkin, Zachariah
Ali, Mannan
Burnell, Gavin
Barker, Joseph
Hickey, B J
Cespedes, Oscar
Strongly Correlated Electrons
Frustrated Kondo spin lattice (KSL) systems away from the antiferromagnetic (AFM) ground state have been found to display strange metal behaviour. A signature of strange metals in correlated systems is large Nernst response. Metallo-molecular interfaces of supramolecular lattices have been demonstrated as 2D KSL systems in STM studies. Here going beyond STM experiments we report a frustrated AFM state on molecular interfaces of Pt(111) and Pt(111)/Co films with around room temperature spin freezing transitions. Near these transitions we measure an anomalous Nernst coefficient of at least 3 $μ$V/K.
title Probing frustrated metallo-molecular spin Kondo lattice interfaces through anomalous Nernst effect
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2510.04824