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Main Authors: Besley, Luke, Jørgensen, P. S., Diaz, A., Detlefs, C., De Angelis, S., Carlsen, M., Chang, B., Silvestre, C., Andreasen, J. W.
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2510.06877
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author Besley, Luke
Jørgensen, P. S.
Diaz, A.
Detlefs, C.
De Angelis, S.
Carlsen, M.
Chang, B.
Silvestre, C.
Andreasen, J. W.
author_facet Besley, Luke
Jørgensen, P. S.
Diaz, A.
Detlefs, C.
De Angelis, S.
Carlsen, M.
Chang, B.
Silvestre, C.
Andreasen, J. W.
contents Coherent imaging techniques such as ptychography offer powerful capabilities for 3D resolution of nanoscale structures. By application in grazing incidence, such techniques may achieve exceptional surface sensitivity as demonstrated by grazing incidence small angle scattering. This requires however an extension of the conventional analysis based on the Distorted Wave Born Approximation which is typically limited to stratified-layer models and statistical descriptions of in-plane structures. The prevailing implementations of reconstruction algorithms for ptychography based on the projection approximation fails to capture the significant multiple scattering that occurs in grazing incidence. We present a ptychographic reconstruction framework that replaces the single-scattering model with a multislice wave-propagation formalism tailored to grazing incidence. The framework supports simultaneous phase retrieval and reconstruction, and can incorporate multiple incidence angles, multiple rotation angles, and flexible experimental geometries into a single inversion. Reconstructions can be initialized from a random guess without strong structural priors, enabling the recovery of complex surface and near-surface nanostructures. This reconstruction framework is applied to both experimental and simulated datasets, demonstrating its versatility.
format Preprint
id arxiv_https___arxiv_org_abs_2510_06877
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Versatile 3D reconstruction framework for hard X-ray grazing incidence imaging of nanostructures
Besley, Luke
Jørgensen, P. S.
Diaz, A.
Detlefs, C.
De Angelis, S.
Carlsen, M.
Chang, B.
Silvestre, C.
Andreasen, J. W.
Optics
Coherent imaging techniques such as ptychography offer powerful capabilities for 3D resolution of nanoscale structures. By application in grazing incidence, such techniques may achieve exceptional surface sensitivity as demonstrated by grazing incidence small angle scattering. This requires however an extension of the conventional analysis based on the Distorted Wave Born Approximation which is typically limited to stratified-layer models and statistical descriptions of in-plane structures. The prevailing implementations of reconstruction algorithms for ptychography based on the projection approximation fails to capture the significant multiple scattering that occurs in grazing incidence. We present a ptychographic reconstruction framework that replaces the single-scattering model with a multislice wave-propagation formalism tailored to grazing incidence. The framework supports simultaneous phase retrieval and reconstruction, and can incorporate multiple incidence angles, multiple rotation angles, and flexible experimental geometries into a single inversion. Reconstructions can be initialized from a random guess without strong structural priors, enabling the recovery of complex surface and near-surface nanostructures. This reconstruction framework is applied to both experimental and simulated datasets, demonstrating its versatility.
title Versatile 3D reconstruction framework for hard X-ray grazing incidence imaging of nanostructures
topic Optics
url https://arxiv.org/abs/2510.06877