Surface band-selective moiré effect induces flat band in mixed-dimensional heterostructures

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Hauptverfasser: Yu, Shuming, Fu, Zhentao, Qin, Dingkun, Li, Enting, Zhong, Hao, Wang, Xingzhe, Zhao, Keming, Mo, Shangkun, Wan, Qiang, Li, Yiwei, Li, Jie, Zhong, Jianxin, Ding, Hong, Xu, Nan
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Veröffentlicht: 2025
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author Yu, Shuming
Fu, Zhentao
Qin, Dingkun
Li, Enting
Zhong, Hao
Wang, Xingzhe
Zhao, Keming
Mo, Shangkun
Wan, Qiang
Li, Yiwei
Li, Jie
Zhong, Jianxin
Ding, Hong
Xu, Nan
author_facet Yu, Shuming
Fu, Zhentao
Qin, Dingkun
Li, Enting
Zhong, Hao
Wang, Xingzhe
Zhao, Keming
Mo, Shangkun
Wan, Qiang
Li, Yiwei
Li, Jie
Zhong, Jianxin
Ding, Hong
Xu, Nan
contents In this work, we reveal a curious type of moiré effect that selectively modifies the surface states of bulk crystal. We synthesize mixed-dimensional heterostructures consisting of a noble gas monolayer grow on the surface of bulk Bi(111), and determine the electronic structure of the heterostructures using angle-resolved photoemission spectroscopy. We directly observe moiré replicas of the Bi(111) surface states, while the bulk states remain barely changed. Meanwhile, we achieve control over the moiré period in the range of 25 Å to 80 Å by selecting monolayers of different noble gases and adjusting the annealing temperature. At large moiré periods, we observe hybridization between the surface band replicas, which leads to the formation of a correlated flat band. Our results serve as a bridge for understanding the moiré modulation effect from 2D to 3D systems, and provide a feasible approach for the realization of correlated phenomena through the engineering of surface states via moiré effects.
format Preprint
id arxiv_https___arxiv_org_abs_2510_07704
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Surface band-selective moiré effect induces flat band in mixed-dimensional heterostructures
Yu, Shuming
Fu, Zhentao
Qin, Dingkun
Li, Enting
Zhong, Hao
Wang, Xingzhe
Zhao, Keming
Mo, Shangkun
Wan, Qiang
Li, Yiwei
Li, Jie
Zhong, Jianxin
Ding, Hong
Xu, Nan
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
In this work, we reveal a curious type of moiré effect that selectively modifies the surface states of bulk crystal. We synthesize mixed-dimensional heterostructures consisting of a noble gas monolayer grow on the surface of bulk Bi(111), and determine the electronic structure of the heterostructures using angle-resolved photoemission spectroscopy. We directly observe moiré replicas of the Bi(111) surface states, while the bulk states remain barely changed. Meanwhile, we achieve control over the moiré period in the range of 25 Å to 80 Å by selecting monolayers of different noble gases and adjusting the annealing temperature. At large moiré periods, we observe hybridization between the surface band replicas, which leads to the formation of a correlated flat band. Our results serve as a bridge for understanding the moiré modulation effect from 2D to 3D systems, and provide a feasible approach for the realization of correlated phenomena through the engineering of surface states via moiré effects.
title Surface band-selective moiré effect induces flat band in mixed-dimensional heterostructures
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2510.07704