Magnetic-Field Control of Tomonaga-Luttinger Liquids in Ta2Pd3Te5 Edge States

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Main Authors: Wang, Xingchen Guo Anqi, Deng, Xiutong, Li, Yupeng, Li, Guoan, Zhang, Zhiyuan, Shi, Xiaofan, Deng, Xiao, Dou, Ziwei, Liu, Guangtong, Qu, Fanming, Wang, Zhijun, Qian, Tian, Shi, Youguo, Lu, Li, Shen, Jie
Format: Preprint
Published: 2025
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author Wang, Xingchen Guo Anqi
Deng, Xiutong
Li, Yupeng
Li, Guoan
Zhang, Zhiyuan
Shi, Xiaofan
Deng, Xiao
Dou, Ziwei
Liu, Guangtong
Qu, Fanming
Wang, Zhijun
Qian, Tian
Shi, Youguo
Lu, Li
Shen, Jie
author_facet Wang, Xingchen Guo Anqi
Deng, Xiutong
Li, Yupeng
Li, Guoan
Zhang, Zhiyuan
Shi, Xiaofan
Deng, Xiao
Dou, Ziwei
Liu, Guangtong
Qu, Fanming
Wang, Zhijun
Qian, Tian
Shi, Youguo
Lu, Li
Shen, Jie
contents Ta2Pd3Te5 is a quasi-one-dimensional transition-metal telluride whose heavy atoms endow the material with strong spin-orbit coupling, while the Fermi level inside the bulk gap makes the low-energy electronic structure highly tunable.Theory and early experiments have already identified a wealth of emergent phases in this platform: an excitonic insulator driven by electron-hole binding, a second-order topological insulator protected by crystalline symmetry, a potential topological-protected quantum-spin-Hall edge, and proximity-induced edge supercurrents when coupled to a conventional s-wave superconductor. These properties make it a promising platform for hosting Majorana zero modes and quantum computation, provided that time-reversal symmetry can be broken by a Zeeman gap. In this work, we demonstrate that the one-dimensional edge channels of exfoliated Ta2Pd3Te5 host a robust and tunable Tomonaga-Luttinger liquid by electrostatic gating because it shifts the chemical potential across the bulk gap without changing the gap size. More importantly, the application of a magnetic field introduces a Zeeman gap that systematically increases the TLL power-law exponent alpha. Furthermore, rotating the field reveals a pronounced twofold anisotropy--alpha is maximal for a field parallel to the edge and minimal for a perpendicular orientation--originating from an orientation-dependent edge g-factor that is likely amplified by quantum-confinement-induced orbital-angular-moment quenching. The existence of gate-tunable edge supercurrents together with the field-controlled Zeeman gap provides a direct route to break time-reversal symmetry in a particle-hole-symmetric superconducting gap and thus to engineer a topological superconducting phase, paving the way towards Majorana-based quantum devices.
format Preprint
id arxiv_https___arxiv_org_abs_2510_07973
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Magnetic-Field Control of Tomonaga-Luttinger Liquids in Ta2Pd3Te5 Edge States
Wang, Xingchen Guo Anqi
Deng, Xiutong
Li, Yupeng
Li, Guoan
Zhang, Zhiyuan
Shi, Xiaofan
Deng, Xiao
Dou, Ziwei
Liu, Guangtong
Qu, Fanming
Wang, Zhijun
Qian, Tian
Shi, Youguo
Lu, Li
Shen, Jie
Mesoscale and Nanoscale Physics
Materials Science
Ta2Pd3Te5 is a quasi-one-dimensional transition-metal telluride whose heavy atoms endow the material with strong spin-orbit coupling, while the Fermi level inside the bulk gap makes the low-energy electronic structure highly tunable.Theory and early experiments have already identified a wealth of emergent phases in this platform: an excitonic insulator driven by electron-hole binding, a second-order topological insulator protected by crystalline symmetry, a potential topological-protected quantum-spin-Hall edge, and proximity-induced edge supercurrents when coupled to a conventional s-wave superconductor. These properties make it a promising platform for hosting Majorana zero modes and quantum computation, provided that time-reversal symmetry can be broken by a Zeeman gap. In this work, we demonstrate that the one-dimensional edge channels of exfoliated Ta2Pd3Te5 host a robust and tunable Tomonaga-Luttinger liquid by electrostatic gating because it shifts the chemical potential across the bulk gap without changing the gap size. More importantly, the application of a magnetic field introduces a Zeeman gap that systematically increases the TLL power-law exponent alpha. Furthermore, rotating the field reveals a pronounced twofold anisotropy--alpha is maximal for a field parallel to the edge and minimal for a perpendicular orientation--originating from an orientation-dependent edge g-factor that is likely amplified by quantum-confinement-induced orbital-angular-moment quenching. The existence of gate-tunable edge supercurrents together with the field-controlled Zeeman gap provides a direct route to break time-reversal symmetry in a particle-hole-symmetric superconducting gap and thus to engineer a topological superconducting phase, paving the way towards Majorana-based quantum devices.
title Magnetic-Field Control of Tomonaga-Luttinger Liquids in Ta2Pd3Te5 Edge States
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2510.07973