Relationship among Structural, Disordered, Magnetism and Band Topology in MnSb2Te4(Sb2Te3)n Family

Fuente: arXiv
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Autori principali: Xi, Ming, Zhang, Yuchong, Zhou, Wenju, Chen, Famin, Jia, Donghan, Gou, Huiyang, Qian, Tian, Lei, Hechang
Natura: Preprint
Pubblicazione: 2025
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author Xi, Ming
Zhang, Yuchong
Zhou, Wenju
Chen, Famin
Jia, Donghan
Gou, Huiyang
Qian, Tian
Lei, Hechang
author_facet Xi, Ming
Zhang, Yuchong
Zhou, Wenju
Chen, Famin
Jia, Donghan
Gou, Huiyang
Qian, Tian
Lei, Hechang
contents Interplay between topology and magnetism induces various exotic quantum phenomena, with magnetic topological insulators (MTIs) serving as a prominent example due to their ability to host the quantum anomalous Hall effect (QAHE). However, the realization of QAHE at higher temperature approaching magnetic-transition-temperature remains a significant challenge, primarily due to the scarcity of suitable material platforms and limited understanding of the intricate relationships between band topology, magnetism, and defects. Here, we report a comprehensive investigation of MnSb2Te4(Sb2Te3)n (n = 0 - 5) single crystals, including the discovery of novel MnSb8Te13 pure phase. Experimental measurements confirm that MnSb8Te13 exhibits ferromagnetism and features topologically nontrivial electronic structures, characterized by a Dirac point located further from the conduction band and a possible larger bulk gap compared to MnBi2Te4(Bi2Te3)n (n = 0 - 3). Moreover, we systematically analyze the relationship between structure, magnetism, topology, and disorder within Mn(Sb, Bi)2Te4((Sb, Bi)2Te3)n family. Present work will shed light on the exploration of potential platforms capable of achieving QAHE near magnetic transition temperature, offering new directions for advancing topological quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2510_09973
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Relationship among Structural, Disordered, Magnetism and Band Topology in MnSb2Te4(Sb2Te3)n Family
Xi, Ming
Zhang, Yuchong
Zhou, Wenju
Chen, Famin
Jia, Donghan
Gou, Huiyang
Qian, Tian
Lei, Hechang
Materials Science
Strongly Correlated Electrons
Interplay between topology and magnetism induces various exotic quantum phenomena, with magnetic topological insulators (MTIs) serving as a prominent example due to their ability to host the quantum anomalous Hall effect (QAHE). However, the realization of QAHE at higher temperature approaching magnetic-transition-temperature remains a significant challenge, primarily due to the scarcity of suitable material platforms and limited understanding of the intricate relationships between band topology, magnetism, and defects. Here, we report a comprehensive investigation of MnSb2Te4(Sb2Te3)n (n = 0 - 5) single crystals, including the discovery of novel MnSb8Te13 pure phase. Experimental measurements confirm that MnSb8Te13 exhibits ferromagnetism and features topologically nontrivial electronic structures, characterized by a Dirac point located further from the conduction band and a possible larger bulk gap compared to MnBi2Te4(Bi2Te3)n (n = 0 - 3). Moreover, we systematically analyze the relationship between structure, magnetism, topology, and disorder within Mn(Sb, Bi)2Te4((Sb, Bi)2Te3)n family. Present work will shed light on the exploration of potential platforms capable of achieving QAHE near magnetic transition temperature, offering new directions for advancing topological quantum materials.
title Relationship among Structural, Disordered, Magnetism and Band Topology in MnSb2Te4(Sb2Te3)n Family
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2510.09973