Anisotropic self-assembly of soft particles mediated by elliptically polarized AC fields

Fuente: arXiv
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Autores principales: Estanislau, Carlos Eduardo, Colla, Thiago, Likos, Christos N.
Formato: Preprint
Publicado: 2025
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author Estanislau, Carlos Eduardo
Colla, Thiago
Likos, Christos N.
author_facet Estanislau, Carlos Eduardo
Colla, Thiago
Likos, Christos N.
contents Attractive dipole interactions can be induced between equally charged soft nanoparticles under the influence of AC electric fields. The combination of charge repulsion and dipole attraction, along with different screening responses from an underlying electrolyte, lead to complex aggregations ranging from chain-like formation for linear polarizations to isotropic planar structures in the case of circular polarizations. In this work, we analyze the role of varying field anisotropies in these self-assembled structures. To this end, the formalism previously developed for the coarse-grained interactions of soft particles in the presence of linear [T.~Colla {\it et al.}, ACS Nano {\bf 12}, 4321-4337 (2018)] and circular [M.~Reich {\it et al.}, Soft Matter {\bf 21}, 1516-1528 (2025)] field polarizations is naturally extended to incorporate elliptical polarizations of arbitrary asymmetries. A rich variety of self-assembly formations is found at intermediate field anisotropies, thus bridging the gap between linear and circular field-induced self-assembly scenarios.
format Preprint
id arxiv_https___arxiv_org_abs_2510_13642
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Anisotropic self-assembly of soft particles mediated by elliptically polarized AC fields
Estanislau, Carlos Eduardo
Colla, Thiago
Likos, Christos N.
Soft Condensed Matter
Attractive dipole interactions can be induced between equally charged soft nanoparticles under the influence of AC electric fields. The combination of charge repulsion and dipole attraction, along with different screening responses from an underlying electrolyte, lead to complex aggregations ranging from chain-like formation for linear polarizations to isotropic planar structures in the case of circular polarizations. In this work, we analyze the role of varying field anisotropies in these self-assembled structures. To this end, the formalism previously developed for the coarse-grained interactions of soft particles in the presence of linear [T.~Colla {\it et al.}, ACS Nano {\bf 12}, 4321-4337 (2018)] and circular [M.~Reich {\it et al.}, Soft Matter {\bf 21}, 1516-1528 (2025)] field polarizations is naturally extended to incorporate elliptical polarizations of arbitrary asymmetries. A rich variety of self-assembly formations is found at intermediate field anisotropies, thus bridging the gap between linear and circular field-induced self-assembly scenarios.
title Anisotropic self-assembly of soft particles mediated by elliptically polarized AC fields
topic Soft Condensed Matter
url https://arxiv.org/abs/2510.13642