Structural origin of resonant diffraction in RuO$_2$

Fuente: arXiv
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Hauptverfasser: Occhialini, Connor A, Nelson, Christie, Bombardi, Alessandro, Fan, Shiyu, Acevedo-Esteves, Raul, Comin, Riccardo, Basov, Dmitri N, Musashi, Maki, Kawasaki, Masashi, Uchida, Masaki, You, Hoydoo, Mitchell, John, Bisogni, Valentina, Mazzoli, Claudio, Pelliciari, Jonathan
Format: Preprint
Veröffentlicht: 2025
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author Occhialini, Connor A
Nelson, Christie
Bombardi, Alessandro
Fan, Shiyu
Acevedo-Esteves, Raul
Comin, Riccardo
Basov, Dmitri N
Musashi, Maki
Kawasaki, Masashi
Uchida, Masaki
You, Hoydoo
Mitchell, John
Bisogni, Valentina
Mazzoli, Claudio
Pelliciari, Jonathan
author_facet Occhialini, Connor A
Nelson, Christie
Bombardi, Alessandro
Fan, Shiyu
Acevedo-Esteves, Raul
Comin, Riccardo
Basov, Dmitri N
Musashi, Maki
Kawasaki, Masashi
Uchida, Masaki
You, Hoydoo
Mitchell, John
Bisogni, Valentina
Mazzoli, Claudio
Pelliciari, Jonathan
contents We report Ru L$_3$-edge resonant X-ray diffraction studies on single crystal and (001) epitaxial films of RuO$_2$. We investigate the distinct $\mathbf{Q} = (100)$ and $(001)$ reflections as a function of incident energy, azimuthal angle, and temperature. The results show that the observed resonant diffraction in RuO$_2$ is fully consistent with a resonant charge anisotropy signal of structural origin permitted by the parent (non-magnetic) rutile $P4_2/mnm$ space group. These results significantly constrain the magnetic contribution to the resonant diffraction signal and indicate the unlikely existence of $\mathbf{k} = 0$ antiferromagnetic order in RuO$_2$.
format Preprint
id arxiv_https___arxiv_org_abs_2510_13767
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Structural origin of resonant diffraction in RuO$_2$
Occhialini, Connor A
Nelson, Christie
Bombardi, Alessandro
Fan, Shiyu
Acevedo-Esteves, Raul
Comin, Riccardo
Basov, Dmitri N
Musashi, Maki
Kawasaki, Masashi
Uchida, Masaki
You, Hoydoo
Mitchell, John
Bisogni, Valentina
Mazzoli, Claudio
Pelliciari, Jonathan
Strongly Correlated Electrons
We report Ru L$_3$-edge resonant X-ray diffraction studies on single crystal and (001) epitaxial films of RuO$_2$. We investigate the distinct $\mathbf{Q} = (100)$ and $(001)$ reflections as a function of incident energy, azimuthal angle, and temperature. The results show that the observed resonant diffraction in RuO$_2$ is fully consistent with a resonant charge anisotropy signal of structural origin permitted by the parent (non-magnetic) rutile $P4_2/mnm$ space group. These results significantly constrain the magnetic contribution to the resonant diffraction signal and indicate the unlikely existence of $\mathbf{k} = 0$ antiferromagnetic order in RuO$_2$.
title Structural origin of resonant diffraction in RuO$_2$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2510.13767