Splitting Isotope Shift in the $1s2p\,^3\!P_{0,1,2}$ Fine-Structure Triplet in $^{12,13,14}$C$^{4+}$: Experiment and Theory

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Main Authors: Müller, Patrick, König, Kristian, Burbach, Emily, Drake, Gordon W. F., Imgram, Phillip, Maaß, Bernhard, Maggio, Titamarie M., Nörtershäuser, Wilfried, Spahn, Julien
Format: Preprint
Published: 2025
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author Müller, Patrick
König, Kristian
Burbach, Emily
Drake, Gordon W. F.
Imgram, Phillip
Maaß, Bernhard
Maggio, Titamarie M.
Nörtershäuser, Wilfried
Spahn, Julien
author_facet Müller, Patrick
König, Kristian
Burbach, Emily
Drake, Gordon W. F.
Imgram, Phillip
Maaß, Bernhard
Maggio, Titamarie M.
Nörtershäuser, Wilfried
Spahn, Julien
contents We report measurements and theoretical calculations of the fine-structure splittings in all three $1s2s\,^3\!S_1\rightarrow\,1s2p\,^3\!P_{0,1,2}$ transitions in the heliumlike systems of the isotopes $^{12,13,14}$C. The metastable triplet state was efficiently populated in an electron beam ion source and the C$^{4+}$ ions were electrostatically accelerated to 50\,keV to perform collinear laser spectroscopy. From the determined transition frequencies, the splitting isotope shift (SIS), i.e., the difference in fine-structure splittings between different isotopes of the same element, was extracted. In the SIS, theoretical uncertainties due to higher-order quantum electrodynamic corrections are strongly suppressed since they are independent of both nuclear mass and the fine-structure quantum number $J$ in lowest order. Comparison with theory provides an important test of experimental accuracy, particularly in the $^{13}$C$^{4+}$ case, for which the nuclear spin leads to hyperfine-induced fine-structure mixing. At the same time, the even-even isotopes $^{12,14}$C$^{4+}$ without nuclear spin can be used to confirm theory. Theoretical values of the SIS are given for all the heliumlike ions with $2\le Z\le 10$.
format Preprint
id arxiv_https___arxiv_org_abs_2510_13779
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Splitting Isotope Shift in the $1s2p\,^3\!P_{0,1,2}$ Fine-Structure Triplet in $^{12,13,14}$C$^{4+}$: Experiment and Theory
Müller, Patrick
König, Kristian
Burbach, Emily
Drake, Gordon W. F.
Imgram, Phillip
Maaß, Bernhard
Maggio, Titamarie M.
Nörtershäuser, Wilfried
Spahn, Julien
Atomic Physics
We report measurements and theoretical calculations of the fine-structure splittings in all three $1s2s\,^3\!S_1\rightarrow\,1s2p\,^3\!P_{0,1,2}$ transitions in the heliumlike systems of the isotopes $^{12,13,14}$C. The metastable triplet state was efficiently populated in an electron beam ion source and the C$^{4+}$ ions were electrostatically accelerated to 50\,keV to perform collinear laser spectroscopy. From the determined transition frequencies, the splitting isotope shift (SIS), i.e., the difference in fine-structure splittings between different isotopes of the same element, was extracted. In the SIS, theoretical uncertainties due to higher-order quantum electrodynamic corrections are strongly suppressed since they are independent of both nuclear mass and the fine-structure quantum number $J$ in lowest order. Comparison with theory provides an important test of experimental accuracy, particularly in the $^{13}$C$^{4+}$ case, for which the nuclear spin leads to hyperfine-induced fine-structure mixing. At the same time, the even-even isotopes $^{12,14}$C$^{4+}$ without nuclear spin can be used to confirm theory. Theoretical values of the SIS are given for all the heliumlike ions with $2\le Z\le 10$.
title Splitting Isotope Shift in the $1s2p\,^3\!P_{0,1,2}$ Fine-Structure Triplet in $^{12,13,14}$C$^{4+}$: Experiment and Theory
topic Atomic Physics
url https://arxiv.org/abs/2510.13779